ArticleNature nanotechnology2021
Intermolecular conical intersections in molecular aggregates.
Article in Nature nanotechnology, 2021. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Direct Observation of Franck-Condon Stimulated Emission and Sub-20 fs Relaxation in Photoexcited Flavins.The journal of physical chemistry letters · 2026Article
- Vibronically assisted sub-cycle charge transfer at a non-fullerene acceptor heterojunction.Nature communications · 2026Article
- Signatures of Antisymmetric Vibrations in the Ultrafast Dynamics of Quadrupolar Dyes.The journal of physical chemistry letters · 2026Article
- Turning Stress Into Signal: Mechanochromic Materials in Commodity and Technologically Relevant Polymers.Chemistry, an Asian journal · 2026Review
- Topological classification of cycloadditions occurring on-surface and in the solid-state.Communications chemistry · 2025Article
- Vibronic coupling-driven symmetry breaking and solvation in the photoexcited dynamics of quadrupolar dyes.Nature chemistry · 2025Article
- Creating a designer cyanobacterial ecosystem for the sustainable production of biomass rich in sun-protecting compounds: mycosporine-like amino acids and scytonemin.Archives of microbiology · 2025Review
- Machine learning photodynamics decode multiple singlet fission channels in pentacene crystal.Nature communications · 2025Article
- Ultrafast Time-Domain Spectroscopy Reveals Coherent Vibronic Couplings upon Electronic Excitation in Crystalline Organic Thin Films.The journal of physical chemistry letters · 2024Article
- Unveiling Multiquantum Excitonic Correlations in Push-Pull Polymer Semiconductors.The journal of physical chemistry letters · 2024Article
- Plasmon mediated coherent population oscillations in molecular aggregates.Nature communications · 2023Article
- Intermolecular-Type Conical Intersections in Benzene Dimer.International journal of molecular sciences · 2023Article
- Mixing of Excitons in Nanostructures Based on a Perylene Dye with CdTe Quantum Dots.Materials (Basel, Switzerland) · 2023Article
Corrections and comments
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Authors and funding
15 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Conical intersections (CoIns) of multidimensional potential energy surfaces are ubiquitous in nature and control pathways and yields of many photo-initiated intramolecular processes. Such topologies can be potentially involved in the energy transport in aggregated molecules or polymers but are yet to be uncovered. Here, using ultrafast two-dimensional electronic spectroscopy (2DES), we reveal the existence of intermolecular CoIns in molecular aggregates relevant for photovoltaics. Ultrafast, sub-10-fs 2DES tracks the coherent motion of a vibrational wave packet on an optically bright state and its abrupt transition into a dark state via a CoIn after only 40 fs. Non-adiabatic dynamics simulations identify an intermolecular CoIn as the source of these unusual dynamics. Our results indicate that intermolecular CoIns may effectively steer energy pathways in functional nanostructures for optoelectronics.
Identifiers
33199882What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.