Evidence map›Paper›PMID 33199622›Full record

ArticleProceedings of the National Academy of Sciences of the United States of America2020

Stable metal anodes enabled by a labile organic molecule bonded to a reduced graphene oxide aerogel.

Yue Gao, Daiwei Wang, Yun Kyung Shin, Zhifei Yan, Zhuo Han, Ke Wang, Md Jamil Hossain, Shuling Shen, Atif AlZahrani, Adri C T van Duin and 2 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Proceedings of the National Academy of Sciences of the United States of America, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

12 authors.

Yue GaoDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.ORCID https://orcid.org/0000-0001-7559-1288
Daiwei WangDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.
Yun Kyung ShinDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.ORCID https://orcid.org/0000-0001-8198-001X
Zhifei YanDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA 19104.
Zhuo HanSchool of Materials Science and Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China.
Ke WangDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.
Md Jamil HossainDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.ORCID https://orcid.org/0000-0002-8737-2821
Shuling ShenSchool of Materials Science and Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China.
Atif AlZahraniDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.ORCID https://orcid.org/0000-0003-1141-0323
Adri C T van DuinDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802.
Thomas E MalloukDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA 19104.ORCID https://orcid.org/0000-0003-4599-4208
Donghai WangDepartment of Mechanical Engineering, The Pennsylvania State University, University Park, PA 16802; dwang@psu.edu.ORCID https://orcid.org/0000-0001-7261-8510

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Metallic anodes (lithium, sodium, and zinc) are attractive for rechargeable battery technologies but are plagued by an unfavorable metal-electrolyte interface that leads to nonuniform metal deposition and an unstable solid-electrolyte interphase (SEI). Here we report the use of electrochemically labile molecules to regulate the electrochemical interface and guide even lithium deposition and a stable SEI. The molecule, benzenesulfonyl fluoride, was bonded to the surface of a reduced graphene oxide aerogel. During metal deposition, this labile molecule not only generates a metal-coordinating benzenesulfonate anion that guides homogeneous metal deposition but also contributes lithium fluoride to the SEI to improve Li surface passivation. Consequently, high-efficiency lithium deposition with a low nucleation overpotential was achieved at a high current density of 6.0 mA cm

Indexed as

electrochemical interfacefunctionalized reduced graphene oxidemetallic anodessolid–electrolyte interphase

Identifiers

PMID33199622
PMCPMC7720105

What OpenQuestion holds

Textmetadata
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.