ArticleMacromolecules2020
Glass Transition of Disentangled and Entangled Polymer Melts: Single-Chain-Nanoparticles Approach.
Article in Macromolecules, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed.
- A Biodegradable Radical Polymer Enables High-Performance, Physically Transient Organic Memory.Angewandte Chemie (International ed. in English) · 2025Article
- High-Speed Electrospinning of Ethyl Cellulose Nanofibers via Taylor Cone Optimization.ACS applied engineering materials · 2024Article
- Viscoelastic and antimicrobial dental care bioplastic with recyclable life cycle.Nature communications · 2024Article
- Electrostimulable polymeric films with hyaluronic acid and lipid nanoparticles for simultaneous topical delivery of macromolecules and lipophilic drugs.Drug delivery and translational research · 2024Article
- Exploring the Processing Potential of Polylactic Acid, Polyhydroxyalkanoate, and Poly(butylene succinate-Polymers · 2024Article
- Synthesis of ultra-high molecular weight homo- and copolymers via an ultrasonic emulsion process with a fast rate.Communications chemistry · 2024Article
- Entanglement-Stabilized Nanoporous Polymer Films Made by Mechanical Deformation.Macromolecules · 2024Article
- Free Standing Dry and Stable Nanoporous Polymer Films Made through Mechanical Deformation.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Structure and Mechanical Properties of a Porous Polymer Material via Molecular Dynamics Simulations.Polymers · 2023Article
- Collective Motions and Mechanical Response of a Bulk of Single-Chain Nano-Particles Synthesized by Click-Chemistry.Polymers · 2020Article
Corrections and comments
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Authors and funding
9 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
We study the effect of entanglements on the glass transition of high molecular weight polymers, by the comparison of single-chain nanoparticles (SCNPs) and equilibrated melts of high-molecular weight polystyrene of identical molecular weight. SCNPs were prepared by electrospraying technique and characterized using scanning electron microscopy and atomic force microscopy techniques. Differential scanning calorimetry, Brillouin light spectroscopy, and rheological experiments around the glass transition were compared. In parallel, entangled and disentangled polymer melts were also compared under cooling from molecular dynamics simulations based on a bead-spring polymer model. While experiments suggest a small decrease in the glass transition temperature of films of nanoparticles in comparison to entangled melts, simulations do not observe any significant difference, despite rather different chain conformations.
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Registered trials
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