ArticleNature communications2020
Excess-entropy scaling in supercooled binary mixtures.
Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Influence of nuclear quantum effects on metastable states of warm dense hydrogen.Scientific reports · 2026Article
- Unifying dynamics of glass-forming liquids by crystallization temperature.National science review · 2025Article
- Entropy scaling for diffusion coefficients in fluid mixtures.Nature communications · 2025Article
- A Picture is Worth a Thousand Timesteps: Excess Entropy Scaling for Rapid Estimation of Diffusion Coefficients in Molecular-Dynamics Simulations of Fluids.Journal of chemical theory and computation · 2024Article
- Mutual Diffusivities of Mixtures of Carbon Dioxide and Hydrogen and Their Solubilities in Brine: Insight from Molecular Simulations.Industrial & engineering chemistry research · 2024Article
- Crossover from gas-like to liquid-like molecular diffusion in a simple supercritical fluid.Nature communications · 2024Article
- Entropy Scaling of Molecular Dynamics in a Prototypical Anisotropic Model near the Glass Transition.The journal of physical chemistry. B · 2023Article
- Connection between water's dynamical and structural properties: Insights from ab initio simulations.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Pressing matter: why are ionic liquids so viscous?Chemical science · 2022Article
- Vitrification of octonary perylene mixtures with ultralow fragility.Science advances · 2021Article
- Diffusion in dense supercritical methane from quasi-elastic neutron scattering measurements.Nature communications · 2021Article
- Theoretical Estimate of the Glass Transition Line of Yukawa One-Component Plasmas.Molecules (Basel, Switzerland) · 2021Article
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Authors and funding
3 authors.
Funding
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Abstract
Transport coefficients, such as viscosity or diffusion coefficient, show significant dependence on density or temperature near the glass transition. Although several theories have been proposed for explaining this dynamical slowdown, the origin remains to date elusive. We apply here an excess-entropy scaling strategy using molecular dynamics computer simulations and find a quasiuniversal, almost composition-independent, relation for binary mixtures, extending eight orders of magnitude in viscosity or diffusion coefficient. Metallic alloys are also well captured by this relation. The excess-entropy scaling predicts a quasiuniversal breakdown of the Stokes-Einstein relation between viscosity and diffusion coefficient in the supercooled regime. Additionally, we find evidence that quasiuniversality extends beyond binary mixtures, and that the origin is difficult to explain using existing arguments for single-component quasiuniversality.
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