ArticleChemistry (Weinheim an der Bergstrasse, Germany)2020
Entropic Mixing Allows Monomeric-Like Absorption in Neat BODIPY Films.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Quantitative Modeling of Polaritonic Emission Using the Source Term Method.The journal of physical chemistry letters · 2025Article
- Merging π-molecular functions achieved through homogeneous liquid-liquid blending of solvent-free alkyl-π liquids.Science and technology of advanced materials · 2025Article
- The Rise and Current Status of Polaritonic Photochemistry and Photophysics.Chemical reviews · 2023Review
- Suppressing non-radiative decay of photochromic organic molecular systems in the strong coupling regime.Physical chemistry chemical physics : PCCP · 2022Article
- Interplay between Polaritonic and Molecular Trap States.The journal of physical chemistry. C, Nanomaterials and interfaces · 2022Article
- Effect of the Aza-N-Bridge and Push-Pull Moieties: A Comparative Study between BODIPYs and Aza-BODIPYs.The Journal of organic chemistry · 2022Article
- Fluorescent Liquid Tetrazines.Molecules (Basel, Switzerland) · 2021Article
- Entropic Mixing Allows Monomeric-Like Absorption in Neat BODIPY Films.Chemistry (Weinheim an der Bergstrasse, Germany) · 2020Article
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Authors and funding
4 authors.
Funding
Abstract
Intermolecular interactions play a crucial role in materials chemistry because they govern thin film morphology. The photophysical properties of films of organic dyes are highly sensitive to the local environment, and a considerable effort has therefore been dedicated to engineering the morphology of organic thin films. Solubilizing side chains can successfully spatially separate chromophores, reducing detrimental intermolecular interactions. However, this strategy is also significantly decreasing achievable dye concentration. Here, five BODIPY derivatives containing small alkyl chains in the α-position were synthesized and photophysically characterized. By blending two or more derivatives, the increase in entropy reduces aggregation and therefore produces films with extreme dye concentration and, at the same time almost solution like absorption properties. Such a film was placed inside an optical cavity and the achieved system was demonstrated to reach the strong exciton-photon coupling regime by virtue of the achieved dye concentration and sharp absorption features of the film.
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