ArticleACS nano2020
Controlling Optically Driven Atomic Migration Using Crystal-Facet Control in Plasmonic Nanocavities.
Article in ACS nano, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 26 papers.
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Who cites it
26 citing papers in PubMed.
- Seeing Beyond RGB Capabilities: Data-Driven and Physics-Guided Broadband Spectral Extrapolation of Plasmonic Nanostructures by Deep Learning.ACS photonics · 2026Article
- Spatiotemporal Raman probing of molecular transport in sub-2-nm plasmonic quasi-2D nanochannels.Science advances · 2026Article
- Near-unity fueling light into a single plasmonic nanocavity.Nanophotonics (Berlin, Germany) · 2025Article
- Alchemically-glazed plasmonic nanocavities using atomic layer metals: controllably synergizing catalysis and plasmonics.Nature communications · 2025Article
- Electronically Perturbed Vibrational Excitations of the Luminescing Stable Blatter Radical.ACS nano · 2025Article
- Controlling Single-Emitter Strong Coupling by Sculpting DNA Dye Scaffolds in NPoM Cavities.The journal of physical chemistry. C, Nanomaterials and interfaces · 2025Article
- Mapping and Optically Writing Nanogap Inhomogeneities in 1-D Extended Plasmonic Nanowire-on-Mirror Cavities.ACS photonics · 2024Article
- Quantifying the ultimate limit of plasmonic near-field enhancement.Nature communications · 2024Article
- Local electric field in nanocavities dictates the vibrational relaxation dynamics of interfacial molecules.Chemical science · 2024Article
- Extensive photochemical restructuring of molecule-metal surfaces under room light.Nature communications · 2024Article
- Metal to insulator transition for conducting polymers in plasmonic nanogaps.Light, science & applications · 2024Article
- Hybrid cavity-antenna architecture for strong and tunable sideband-selective molecular Raman scattering enhancement.Science advances · 2023Article
- Quantum Plasmonics in Sub-Atom-Thick Optical Slots.Nano letters · 2023Article
- Article
- Full Control of Plasmonic Nanocavities Using Gold Decahedra-on-Mirror Constructs with Monodisperse Facets.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Nanoparticle-on-mirror pairs: building blocks for remote spectroscopies.Nanophotonics (Berlin, Germany) · 2022Article
- The Poynting Vector Field Generic Singularities in Resonant Scattering of Plane Linearly Polarized Electromagnetic Waves by Subwavelength Particles.Nanomaterials (Basel, Switzerland) · 2022Article
- Picocavities: a Primer.Nano letters · 2022Article
- Optical suppression of energy barriers in single molecule-metal binding.Science advances · 2022Article
- Integrated Molecular Optomechanics with Hybrid Dielectric-Metallic Resonators.ACS photonics · 2021Article
Corrections and comments
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Plasmonic nanoconstructs are widely exploited to confine light for applications ranging from quantum emitters to medical imaging and biosensing. However, accessing extreme near-field confinement using the surfaces of metallic nanoparticles often induces permanent structural changes from light, even at low intensities. Here, we report a robust and simple technique to exploit crystal facets and their atomic boundaries to prevent the hopping of atoms along and between facet planes. Avoiding X-ray or electron microscopy techniques that perturb these atomic restructurings, we use elastic and inelastic light scattering to resolve the influence of crystal habit. A clear increase in stability is found for {100} facets with steep inter-facet angles, compared to multiple atomic steps and shallow facet curvature on spherical nanoparticles. Avoiding atomic hopping allows Raman scattering on molecules with low Raman cross-section while circumventing effects of charging and adatom binding, even over long measurement times. These nanoconstructs allow the optical probing of dynamic reconstruction in nanoscale surface science, photocatalysis, and molecular electronics.
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