ArticleNature communications2020
Imaging spatiotemporal evolution of molecules and active sites in zeolite catalyst during methanol-to-olefins reaction.
Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Multiscale spatiotemporal heterogeneity of zeolite-catalyzed methanol-to-hydrocarbons reaction.National science review · 2026Review
- Single-molecule neuromorphic device with aJ-level power consumption per switching.Nature communications · 2026Article
- Electrochemical imaging of thermochemical catalysis.Nature catalysis · 2026Article
- Advancements in Understanding the Physicochemical Properties of Reticular Materials: An In Situ and Operando Spectroscopic Perspective.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Article
- Operando Modeling of Zeolite-Catalyzed Reactions Using First-Principles Molecular Dynamics Simulations.ACS catalysis · 2023Review
- Emerging analytical methods to characterize zeolite-based materials.National science review · 2022Review
- Multiscale dynamical cross-talk in zeolite-catalyzed methanol and dimethyl ether conversions.National science review · 2022Article
- Nano-scale insights regarding coke formation in zeolite SSZ-13 subject to the methanol-to-hydrocarbons reaction.Catalysis science & technology · 2022Article
- MAPO-18 Catalysts for the Methanol to Olefins Process: Influence of Catalyst Acidity in a High-Pressure Syngas (CO and HACS catalysis · 2022Article
- Stabilizing the framework of SAPO-34 zeolite toward long-term methanol-to-olefins conversion.Nature communications · 2021Article
- Synergistically enhance confined diffusion by continuum intersecting channels in zeolites.Science advances · 2021Article
- Directed transforming of coke to active intermediates in methanol-to-olefins catalyst to boost light olefins selectivity.Nature communications · 2021Article
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Direct visualization of spatiotemporal evolution of molecules and active sites during chemical transformation in individual catalyst crystal will accelerate the intuitive understanding of heterogeneous catalysis. So far, widespread imaging techniques can only provide limited information either with large probe molecules or in model catalyst of large size, which are beyond the interests of industrial catalysis. Herein, we demonstrate a feasible deep data approach via synergy of multiscale reaction-diffusion simulation and super-resolution structured illumination microscopy to illustrate the dynamical evolution of spatiotemporal distributions of gas molecules, carbonaceous species and acid sites in SAPO-34 zeolite crystals of several micrometers that are typically used in industrial methanol-to-olefins process. The profound insights into the inadequate utilization of activated acid sites and rapid deactivation are unveiled. The notable elucidation of molecular reaction-diffusion process at the scale of single catalyst crystal via this approach opens an interesting method for mechanism study in materials synthesis and catalysis.
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Registered trials
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