Evidence map›Paper›PMID 32532975›Full record

ArticleNature communications2020

Water stable molecular n-doping produces organic electrochemical transistors with high transconductance and record stability.

Alexandra F Paterson, Achilleas Savva, Shofarul Wustoni, Leonidas Tsetseris, Bryan D Paulsen, Hendrik Faber, Abdul Hamid Emwas, Xingxing Chen, Georgios Nikiforidis, Tania C Hidalgo and 6 more

Abstract read
In one paragraph

Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 28 papers.

0numbers the graph read from it
0cells of the map it votes in
28citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

28 citing papers in PubMed.

  1. Article
  2. Structure-Driven Ion Transport in Conjugated Polymers with Crown Ether Side Chains: From the Nano- to Microscale.Chemistry of materials : a publication of the American Chemical Society · 2026
    Article
  3. Article
  4. Article
  5. Counterion-Controlled Photocatalytic Doping of Organic Semiconductors.Advanced materials (Deerfield Beach, Fla.) · 2026
    Article
  6. Article
  7. Article
  8. Review
  9. Review
  10. Article
  11. Review
  12. Organic Electrochemical Transistors for Biomarker Detections.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024
    Review
  13. Article
  14. Article
  15. Article
  16. Article
  17. Article
  18. Article
  19. Article
  20. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

16 authors.

Alexandra F PatersonOrganic Bioelectronics Laboratory, Biological and Environmental Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Achilleas SavvaOrganic Bioelectronics Laboratory, Biological and Environmental Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.ORCID http://orcid.org/0000-0002-0197-0290
Shofarul WustoniOrganic Bioelectronics Laboratory, Biological and Environmental Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.ORCID http://orcid.org/0000-0002-3059-4503
Leonidas TsetserisDepartment of Physics, National Technical University of Athens, Athens, GR-15780, Greece.ORCID http://orcid.org/0000-0002-0330-0813
Bryan D PaulsenDepartment of Biomedical Engineering, Northwestern University, Evanston, IL, 60208, USA.ORCID http://orcid.org/0000-0002-0923-8475
Hendrik FaberKing Abdullah University of Science and Technology (KAUST) Solar Center (KSC), Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Abdul Hamid EmwasCore Labs, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Xingxing ChenKing Abdullah University of Science and Technology (KAUST) Solar Center (KSC), Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Georgios NikiforidisOrganic Bioelectronics Laboratory, Biological and Environmental Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Tania C HidalgoOrganic Bioelectronics Laboratory, Biological and Environmental Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.ORCID http://orcid.org/0000-0001-5299-9539
Maximillian MoserDepartment of Chemistry and Centre for Plastic Electronics, Imperial College London South Kensington, London, SW7 2AZ, UK.
Iuliana Petruta MariaDepartment of Chemistry and Centre for Plastic Electronics, Imperial College London South Kensington, London, SW7 2AZ, UK.
Jonathan RivnayDepartment of Biomedical Engineering, Northwestern University, Evanston, IL, 60208, USA.ORCID http://orcid.org/0000-0002-0602-6485
Iain McCullochKing Abdullah University of Science and Technology (KAUST) Solar Center (KSC), Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia.
Thomas D AnthopoulosKing Abdullah University of Science and Technology (KAUST) Solar Center (KSC), Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia. thomas.anthopoulos@kaust.edu.sa.ORCID http://orcid.org/0000-0002-0978-8813
Sahika InalOrganic Bioelectronics Laboratory, Biological and Environmental Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955-6900, Saudi Arabia. sahika.inal@kaust.edu.sa.ORCID http://orcid.org/0000-0002-1166-1512

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

From established to emergent technologies, doping plays a crucial role in all semiconducting devices. Doping could, theoretically, be an excellent technique for improving repressively low transconductances in n-type organic electrochemical transistors - critical for advancing logic circuits for bioelectronic and neuromorphic technologies. However, the technical challenge is extreme: n-doped polymers are unstable in electrochemical transistor operating environments, air and water (electrolyte). Here, the first demonstration of doping in electron transporting organic electrochemical transistors is reported. The ammonium salt tetra-n-butylammonium fluoride is simply admixed with the conjugated polymer poly(N,N'-bis(7-glycol)-naphthalene-1,4,5,8-bis(dicarboximide)-co-2,2'-bithiophene-co-N,N'-bis(2-octyldodecyl)-naphthalene-1,4,5,8-bis(dicarboximide), and found to act as a simultaneous molecular dopant and morphology-additive. The combined effects enhance the n-type transconductance with improved channel capacitance and mobility. Furthermore, operational and shelf-life stability measurements showcase the first example of water-stable n-doping in a polymer. Overall, the results set a precedent for doping/additives to impact organic electrochemical transistors as powerfully as they have in other semiconducting devices.

Identifiers

PMID32532975
PMCPMC7293298

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.