ArticleNature communications2020
Hot carriers perspective on the nature of traps in perovskites.
Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 28 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
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Who cites it
28 citing papers in PubMed.
- Ultrafast directional hot carrier transfer in bilayer perovskite heterojunctions.Nature communications · 2026Article
- Photophysics of Distinguished Defect States in BiNanophotonics (Berlin, Germany) · 2026Article
- Defect Passivation Strategies in Halide Perovskite Solar Cells and LEDs.ACS energy letters · 2026Review
- Suppressing electron-phonon coupling in perovskite nanoplatelets for efficient pure-red light-emitting diodes with narrow spectral emission.Nature communications · 2026Article
- Sub-µm Hot Carrier Diffusion in 2D MoSSmall methods · 2026Article
- Article
- Temperature-dependent trapping and polaron annihilation on ultrafast time scales in metal-halide perovskites.The journal of physical chemistry letters · 2025Article
- Enhanced Efficiency and Stability of Perovskite Solar Cells Through Neodymium-Doped Upconversion Nanoparticles with TiOMolecules (Basel, Switzerland) · 2025Article
- Multifaceted nature of defect tolerance in halide perovskites and emerging semiconductors.Nature reviews. Chemistry · 2025Review
- NIR Luminescence from Deep-Level Traps in CsPbBrThe journal of physical chemistry letters · 2025Article
- Mechanism of Hot-Carrier Photoluminescence in Sn-Based Perovskites.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Anomalous Polarons in Two-Dimensional Organometallic Perovskite Ferroelectric.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Extending the defect tolerance of halide perovskite nanocrystals to hot carrier cooling dynamics.Nature communications · 2024Article
- Hot Carrier Trapping and It's Influence to the Carrier Diffusion in CsPbBrAdvanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Cation Influence on Hot-Carrier Relaxation in Tin Triiodide Perovskite Thin Films.ACS energy letters · 2024Article
- Alloying metal cations in perovskite nanocrystals is a new route to controlling hot carrier cooling.Light, science & applications · 2023Article
- Carrier multiplication in perovskite solar cells with internal quantum efficiency exceeding 100.Nature communications · 2023Article
- Tailoring Interlayer Charge Transfer Dynamics in 2D Perovskites with Electroactive Spacer Molecules.Journal of the American Chemical Society · 2023Article
- Thermalization and relaxation mediated by phonon management in tin-lead perovskites.Light, science & applications · 2023Article
- Carriers, Quasi-particles, and Collective Excitations in Halide Perovskites.Chemical reviews · 2023Review
Corrections and comments
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Authors and funding
8 authors.
Funding
Abstract
Amongst the many spectacular properties of hybrid lead halide perovskites, their defect tolerance is regarded as the key enabler for a spectrum of high-performance optoelectronic devices that propel perovskites to prominence. However, the plateauing efficiency enhancement of perovskite devices calls into question the extent of this defect tolerance in perovskite systems; an opportunity for perovskite nanocrystals to fill. Through optical spectroscopy and phenomenological modeling based on the Marcus theory of charge transfer, we uncover the detrimental effect of hot carriers trapping in methylammonium lead iodide and bromide nanocrystals. Higher excess energies induce faster carrier trapping rates, ascribed to interactions with shallow traps and ligands, turning these into potent defects. Passivating these traps with the introduction of phosphine oxide ligands can help mitigate hot carrier trapping. Importantly, our findings extend beyond photovoltaics and are relevant for low threshold lasers, light-emitting devices and multi-exciton generation devices.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.