ArticleACS photonics2020
Relevance of the Quadratic Diamagnetic and Self-Polarization Terms in Cavity Quantum Electrodynamics.
Article in ACS photonics, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 49 papers.
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Who cites it
49 citing papers in PubMed.
- Polaritonic Coupled Cluster Theory for Unpolarized Cavities Exploiting Point-Group Symmetry.Journal of chemical theory and computation · 2026Article
- Vibrationally Induced Resonances in Lasing.The journal of physical chemistry letters · 2026Article
- Collectively-Modified Intermolecular Electron Correlations: The Connection of Polaritonic Chemistry and Spin Glass Physics.Chemical reviews · 2026Review
- Polaritonic quantum matter.Nanophotonics (Berlin, Germany) · 2025Review
- Investigating Cavity Quantum Electrodynamics-Enabled Endo/Exo-Selectivities in a Diels-Alder Reaction.The journal of physical chemistry. A · 2025Article
- Description of ultrastrong light-matter interaction through coupled harmonic oscillator models and their connection with cavity-QED Hamiltonians.Nanophotonics (Berlin, Germany) · 2025Article
- Bound polariton states in the Dicke-Ising model.Nanophotonics (Berlin, Germany) · 2025Article
- Molecular Polarizability under Vibrational Strong Coupling.Journal of chemical theory and computation · 2025Article
- Strong Coupling Quantum Electrodynamics Hartree-Fock Response Theory.The journal of physical chemistry. A · 2025Article
- On-demand heralded MIR single-photon source using a cascaded quantum system.Science advances · 2025Article
- Quantum-Electrodynamical Density-Functional Theory Exemplified by the Quantum Rabi Model.The journal of physical chemistry. A · 2025Article
- Density-Functional Theory for the Dicke Hamiltonian.Journal of statistical physics · 2025Article
- Disentangling collective coupling in vibrational polaritons with double quantum coherence spectroscopy.The Journal of chemical physics · 2024Article
- Analytical Evaluation of Ground State Gradients in Quantum Electrodynamics Coupled Cluster Theory.Journal of chemical theory and computation · 2024Article
- Controlling Plasmonic Catalysis via Strong Coupling with Electromagnetic Resonators.Nano letters · 2024Article
- Do Molecular Geometries Change Under Vibrational Strong Coupling?The journal of physical chemistry letters · 2024Article
- Extending the Tavis-Cummings model for molecular ensembles-Exploring the effects of dipole self-energies and static dipole moments.The Journal of chemical physics · 2024Article
- Cavity Quantum Electrodynamics EnablesJournal of the American Chemical Society · 2024Article
- Investigating the collective nature of cavity-modified chemical kinetics under vibrational strong coupling.Nanophotonics (Berlin, Germany) · 2024Article
- Extracting kinetic information from short-time trajectories: relaxation and disorder of lossy cavity polaritons.Nanophotonics (Berlin, Germany) · 2024Article
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4 authors.
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No grant is acknowledged in the PubMed record.
Abstract
Experiments at the interface of quantum optics and chemistry have revealed that strong coupling between light and matter can substantially modify the chemical and physical properties of molecules and solids. While the theoretical description of such situations is usually based on nonrelativistic quantum electrodynamics, which contains quadratic light-matter coupling terms, it is commonplace to disregard these terms and restrict the treatment to purely bilinear couplings. In this work, we clarify the physical origin and the substantial impact of the most common quadratic terms, the diamagnetic and self-polarization terms, and highlight why neglecting them can lead to rather unphysical results. Specifically, we demonstrate their relevance by showing that neglecting these terms leads to the loss of gauge invariance, basis set dependence, disintegration (loss of bound states) of any system in the basis set limit, unphysical radiation of the ground state, and an artificial dependence on the static dipole. Besides providing important guidance for modeling of strongly coupled light-matter systems, the presented results also indicate conditions under which those effects might become accessible.
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