ArticleJournal of the American Chemical Society2020
Enhancing Long-Range Energy Transport in Supramolecular Architectures by Tailoring Coherence Properties.
Article in Journal of the American Chemical Society, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed, 67 citations in OpenAlex.
- Fluorine Positional Isomerism Enables H-Aggregation for High-Performance Semicrystalline Polymer Donors in Organic Solar Cells.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Long-Range Exciton Transport in Anthracene-Based Supramolecular Mesostructures and Its Control by Surface Plasmons.Nano letters · 2026Article
- Programmable Construction of Supramolecular Polymers Achieved in Neutral Lipid Environments.Nature communications · 2026Article
- Template-directed vertical photopolymerization for construction of triphenylamine-based poly(diacetylene) nanofibers.Nature communications · 2026Article
- Ultralong-range exciton transport in submillimeter-scale spherulite film of π-conjugated polymers.Nature communications · 2026Article
- Light-Harvesting Nanomaterials Based on Dyes for Energy Transfer and Amplified Biosensing.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Tuning Exciton Diffusion in Organic Semiconductors through Hybridization with Charge-Transfer Excitations.The journal of physical chemistry letters · 2025Article
- Optical Properties of H-Bonded Heterotriangulene Supramolecular Polymers: Charge-Transfer Excitations Matter.The journal of physical chemistry letters · 2024Article
- Spatial Correlations Drive Long-Range Transport and Trapping of Excitons in Single H-Aggregates: Experiment and Theory.The journal of physical chemistry letters · 2024Article
- Unusual Photophysical Properties of Porphyrin-Based Supramolecular Polymers Unveiled: The Role of Metal Ligands and Side Group Amide Connectivity.The journal of physical chemistry. C, Nanomaterials and interfaces · 2023Article
- Tailoring Enhanced Elasticity of Crystalline Coordination Polymers.Crystal growth & design · 2023Article
- Interplay Between Hydrogen Bonding and Electron Transfer in Mixed Valence Assemblies of Triarylamine Trisamides.Chemistry (Weinheim an der Bergstrasse, Germany) · 2023Article
- Disorder in P3HT Nanoparticles Probed by Optical Spectroscopy on P3HT-The journal of physical chemistry. A · 2021Article
- Construction of Supramolecular Polymers with Different Topologies by Orthogonal Self-Assembly of Cryptand-Paraquat Recognition and Metal Coordination.Molecules (Basel, Switzerland) · 2021Article
- Molecular versus Excitonic Disorder in Individual Artificial Light-Harvesting Systems.Journal of the American Chemical Society · 2020Article
Corrections and comments
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Authors and funding
10 authors at 4 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Efficient long-range energy transport along supramolecular architectures of functional organic molecules is a key step in nature for converting sunlight into a useful form of energy. Understanding and manipulating these transport processes on a molecular and supramolecular scale is a long-standing goal. However, the realization of a well-defined system that allows for tuning morphology and electronic properties as well as for resolution of transport in space and time is challenging. Here we show how the excited-state energy landscape and thus the coherence characteristics of electronic excitations can be modified by the hierarchical level of H-type supramolecular architectures. We visualize, at room temperature, long-range incoherent transport of delocalized singlet excitons on pico- to nanosecond time scales in single supramolecular nanofibers and bundles of nanofibers. Increasing the degree of coherence, i.e., exciton delocalization, via supramolecular architectures enhances exciton diffusivities up to 1 order of magnitude. In particular, we find that single supramolecular nanofibers exhibit the highest diffusivities reported for H-aggregates so far.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.