ArticleChemphyschem : a European journal of chemical physics and physical chemistry2020
Carbon Nanomembranes from Aromatic Carboxylate Precursors.
Article in Chemphyschem : a European journal of chemical physics and physical chemistry, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Electron-Beam-Induced Modification of N-Heterocyclic Carbenes: Carbon Nanomembrane Formation.The journal of physical chemistry letters · 2024Article
- Defect-Healed Carbon Nanomembranes for Enhanced Salt Separation: Scalable Synthesis and Performance.ACS applied materials & interfaces · 2024Article
- Scalable Synthesis of Carbon Nanomembranes from Amorphous Molecular Layers.ACS applied materials & interfaces · 2023Article
- Effect of Electron and Proton Irradiation on Structural and Electronic Properties of Carbon Nanowalls.ACS omega · 2022Article
- Vapor Adsorption Measurements with Two-Dimensional Membranes.Chemphyschem : a European journal of chemical physics and physical chemistry · 2022Article
- Investigation of electron-induced cross-linking of self-assembled monolayers by scanning tunneling microscopy.Beilstein journal of nanotechnology · 2022Article
- Bottom-up synthesis of graphene films hosting atom-thick molecular-sieving apertures.Proceedings of the National Academy of Sciences of the United States of America · 2021Article
- Exploring the fabrication and transfer mechanism of metallic nanostructures on carbon nanomembranes via focused electron beam induced processing.Beilstein journal of nanotechnology · 2021Article
- Carbon Nanomembranes from Aromatic Carboxylate Precursors.Chemphyschem : a European journal of chemical physics and physical chemistry · 2020Article
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Authors and funding
5 authors.
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Abstract
Self-assembled monolayers (SAMs) serve as convenient platform for fabricating carbon nanomembranes (CNMs) of extended lateral dimensions. Highly porous CNMs are emerging as interesting materials for membrane technologies as they exhibit selectivity for water permeation and, owing to their reduced dimensionality, promise increased energy efficiency compared to established systems. In the present study terphenylcarboxylate SAMs, prepared on silver underpotential deposited on Au and irradiated by 100 eV electrons, were successfully converted into free-standing CNMs. Infrared and X-ray photoelectron spectroscopy reveal pronounced chemical changes both of the anchoring carboxylate moiety and the aromatic backbone upon electron irradiation. Permeation studies showed high specificity for water as demonstrated by the separation from tetrahydrofuran. Compared to thiols on gold, the standard CNM precursor system, the carboxylic acid based SAM exhibits equivalent characteristics. This suggests that electron-induced carbonization is insensitive to the particular choice of the anchor moiety and, therefore, the choice of precursor molecules can be extended to the versatile class of aromatic carboxylic acids.
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