ArticleThe journal of physical chemistry letters2020
Polariton Transitions in Femtosecond Transient Absorption Studies of Ultrastrong Light-Molecule Coupling.
Article in The journal of physical chemistry letters, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 32 papers.
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Who cites it
32 citing papers in PubMed, 104 citations in OpenAlex.
- Strong light-matter interactions in hybrid polaritonic systems.Chemical communications (Cambridge, England) · 2026Review
- Long-lived polaritonic coherence and polaron decoupling effects in 2D electronic spectra.Proceedings of the National Academy of Sciences of the United States of America · 2026Article
- Reservoir Dynamics in Vibrational Polaritons Revealed by Detuning-Dependent Ultrafast Spectroscopy.The journal of physical chemistry letters · 2026Article
- Comparing Exciton-Plasmon Couplings in J-Aggregate and TMD-Based Hybrids Using Angle-Resolved Two-Dimensional Electronic Spectroscopy.Nanophotonics (Berlin, Germany) · 2026Article
- Direct Readout of Excited-State Lifetimes in Chlorin Chromophores under Electronic Strong Coupling.Journal of the American Chemical Society · 2026Article
- Phase-Resolved Two-Dimensional Infrared Spectroscopy of Solution-Phase Vibrational Polaritons on Gold Antenna Meta-Surfaces.The journal of physical chemistry letters · 2026Article
- Ultrafast Dynamics of Organic Exciton-Polaritons.Nanophotonics (Berlin, Germany) · 2026Article
- Ultrafast transition from coherent to incoherent polariton nonlinearities in a hybrid 1L-WSNature nanotechnology · 2026Article
- Collectively-Modified Intermolecular Electron Correlations: The Connection of Polaritonic Chemistry and Spin Glass Physics.Chemical reviews · 2026Review
- Perspective on Many-Body Methods for Molecular Polaritonic Systems.Journal of chemical theory and computation · 2025Review
- Excited State Dynamics of COJournal of the American Chemical Society · 2025Article
- Impact of Dark Polariton States on Collective Strong Light-Matter Coupling in Molecules.The journal of physical chemistry letters · 2025Article
- A Complete Active Space Self-Consistent Field Approach for Molecules in QED Environments.Journal of chemical theory and computation · 2025Article
- Efficient cavity-mediated energy transfer between photosynthetic light harvesting complexes from strong to weak coupling regime.Nature communications · 2025Article
- Theory of terahertz pump optical probe spectroscopy of phonon polaritons in noncentrosymmetric systems.npj quantum materials · 2025Article
- Disentangling collective coupling in vibrational polaritons with double quantum coherence spectroscopy.The Journal of chemical physics · 2024Article
- Probing the anharmonicity of vibrational polaritons with double-quantum two-dimensional infrared spectroscopy.Nanophotonics (Berlin, Germany) · 2024Article
- Molecular Polaritons for Chemistry, Photonics and Quantum Technologies.Chemical reviews · 2024Review
- Plasmon mediated coherent population oscillations in molecular aggregates.Nature communications · 2023Article
- The Rise and Current Status of Polaritonic Photochemistry and Photophysics.Chemical reviews · 2023Review
Corrections and comments
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Authors and funding
8 authors at 3 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Strong light-matter coupling is emerging as a fascinating way to tune optical properties and modify the photophysics of molecular systems. In this work, we studied a molecular chromophore under strong coupling with the optical mode of a Fabry-Perot cavity resonant to the first electronic absorption band. Using femtosecond pump-probe spectroscopy, we investigated the transient response of the cavity-coupled molecules upon photoexcitation resonant to the upper and lower polaritons. We identified an excited state absorption from upper and lower polaritons to a state at the energy of the second cavity mode. Quantum mechanical calculations of the many-molecule energy structure of cavity polaritons suggest assignment of this state as a two-particle polaritonic state with optically allowed transitions from the upper and lower polaritons. We provide new physical insight into the role of two-particle polaritonic states in explaining transient signatures in hybrid light-matter coupling systems consistent with analogous many-body systems.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.