ArticleProceedings of the National Academy of Sciences of the United States of America2020
High-throughput, combinatorial synthesis of multimetallic nanoclusters.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 31 papers.
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Who cites it
31 citing papers in PubMed.
- Unveiling the correlation between high-entropy alloy element systems and electrocatalytic activity.National science review · 2026Article
- Post-ageing guided closed-loop discovery of multi-element alloy catalysts for automotive exhaust purification.Nanoscale advances · 2026Article
- Non-Equilibrium Synthesis Methods to Create Metastable and High-Entropy Nanomaterials.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Review
- Prospects of Nanoscience with Nanocrystals: 2025 Edition.ACS nano · 2025Review
- Article
- Precise synthesis of targeted noble metal-based high-entropy alloy nanomaterials.Science advances · 2025Article
- Finely tailoring the local ensembles in heterostructured high entropy alloy catalysts through pulsed annealing.Nature communications · 2025Article
- Modern strategies in classical fields of nanoindentation: Semiconductors, ceramics, and thin films.MRS bulletin · 2025Review
- Electrothermally-Driven Ultrafast Chemical Modulation of Multifunctional Nanocarbon Aerogels.Small (Weinheim an der Bergstrasse, Germany) · 2024Article
- Integrating few-atom layer metal on high-entropy alloys to catalyze nitrate reduction in tandem.Nature communications · 2024Article
- Future prospects of high-entropy alloys as next-generation industrial electrode materials.Chemical science · 2024Review
- Using scalable computer vision to automate high-throughput semiconductor characterization.Nature communications · 2024Article
- Interfacing High-Throughput Electrosynthesis and Mass Spectrometric Analysis of Azines.Analytical chemistry · 2024Article
- Ultrafast micro/nano-manufacturing of metastable materials for energy.National science review · 2024Review
- Automated crystal system identification from electron diffraction patterns using multiview opinion fusion machine learning.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Legion: An Instrument for High-Throughput Electrochemistry.ACS measurement science au · 2023Article
- Transient and general synthesis of high-density and ultrasmall nanoparticles on two-dimensional porous carbon via coordinated carbothermal shock.Nature communications · 2023Article
- High-entropy alloy nanopatterns by prescribed metallization of DNA origami templates.Nature communications · 2023Article
- Surfactant-Free Colloidal Syntheses of Gold-Based Nanomaterials in Alkaline Water and Mono-alcohol Mixtures.Chemistry of materials : a publication of the American Chemical Society · 2023Article
- Machine learning for a sustainable energy future.Nature reviews. Materials · 2023Review
Corrections and comments
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Authors and funding
21 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Multimetallic nanoclusters (MMNCs) offer unique and tailorable surface chemistries that hold great potential for numerous catalytic applications. The efficient exploration of this vast chemical space necessitates an accelerated discovery pipeline that supersedes traditional "trial-and-error" experimentation while guaranteeing uniform microstructures despite compositional complexity. Herein, we report the high-throughput synthesis of an extensive series of ultrafine and homogeneous alloy MMNCs, achieved by 1) a flexible compositional design by formulation in the precursor solution phase and 2) the ultrafast synthesis of alloy MMNCs using thermal shock heating (i.e., ∼1,650 K, ∼500 ms). This approach is remarkably facile and easily accessible compared to conventional vapor-phase deposition, and the particle size and structural uniformity enable comparative studies across compositionally different MMNCs. Rapid electrochemical screening is demonstrated by using a scanning droplet cell, enabling us to discover two promising electrocatalysts, which we subsequently validated using a rotating disk setup. This demonstrated high-throughput material discovery pipeline presents a paradigm for facile and accelerated exploration of MMNCs for a broad range of applications.
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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.