Evidence map›Paper›PMID 32098968›Full record

ArticleNature communications2020

Connecting energetics to dynamics in particle growth by oriented attachment using real-time observations.

Lili Liu, Elias Nakouzi, Maria L Sushko, Gregory K Schenter, Christopher J Mundy, Jaehun Chun, James J De Yoreo

Abstract read
In one paragraph

Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 21 papers.

0numbers the graph read from it
0cells of the map it votes in
21citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

21 citing papers in PubMed.

  1. Article
  2. Imperfect Oriented Attachment of Gold Nanoparticles.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026
    Article
  3. Article
  4. Review
  5. Article
  6. Article
  7. Article
  8. Article
  9. Article
  10. Article
  11. Article
  12. Understanding the mechanisms of anisotropic dissolution in metal oxides by applying radiolysis simulations to liquid-phase TEM.Proceedings of the National Academy of Sciences of the United States of America · 2023
    Article
  13. Article
  14. Article
  15. Article
  16. Particle-based hematite crystallization is invariant to initial particle morphology.Proceedings of the National Academy of Sciences of the United States of America · 2022
    Article
  17. Article
  18. Article
  19. Ion-dependent protein-surface interactions from intrinsic solvent response.Proceedings of the National Academy of Sciences of the United States of America · 2021
    Article
  20. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

7 authors.

Lili Liu *Physical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA.ORCID http://orcid.org/0000-0002-9595-4303
Elias Nakouzi *Physical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA.
Maria L SushkoPhysical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA.ORCID http://orcid.org/0000-0002-7229-7072
Gregory K SchenterPhysical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA.
Christopher J MundyPhysical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA.
Jaehun ChunPhysical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA. Jaehun.Chun@pnnl.gov.ORCID http://orcid.org/0000-0002-2291-6496
James J De YoreoPhysical Sciences Division, Pacific Northwest National Laboratory, Richland, WA, 99352, USA. James.DeYoreo@pnnl.gov.

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

The interplay between crystal and solvent structure, interparticle forces and ensemble particle response dynamics governs the process of crystallization by oriented attachment (OA), yet a quantitative understanding is lacking. Using ZnO as a model system, we combine in situ TEM observations of single particle and ensemble assembly dynamics with simulations of interparticle forces and responses to relate experimentally derived interparticle potentials to the underlying interactions. We show that OA is driven by forces and torques due to a combination of electrostatic ion-solvent correlations and dipolar interactions that act at separations well beyond 5 nm. Importantly, coalignment is achieved before particles reach separations at which strong attractions drive the final jump to contact. The observed barrier to attachment is negligible, while dissipative factors in the quasi-2D confinement of the TEM fluid cell lead to abnormal diffusivities with timescales for rotation much less than for translation, thus enabling OA to dominate.

Identifiers

PMID32098968
PMCPMC7042275

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.