ArticleThe journal of physical chemistry letters2020
Femtosecond Soft-X-ray Absorption Spectroscopy of Liquids with a Water-Window High-Harmonic Source.
Article in The journal of physical chemistry letters, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 20 papers.
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Who cites it
20 citing papers in PubMed.
- Ultrafast Spectroscopy with anACS physical chemistry Au · 2026Article
- Optical kicking of liquid droplets for sample delivery in ultrafast soft X-ray experiments.Journal of synchrotron radiation · 2025Article
- Attosecond spectroscopy of molecular charge transfer uncovers a 1.5-fs delay in population transfer.Nature communications · 2025Article
- Ultrafast spectroscopy of liquids using extreme-ultraviolet to soft-X-ray pulses.Nature reviews. Chemistry · 2025Review
- Electronic dynamics created at conical intersections and its dephasing in aqueous solution.Nature physics · 2025Article
- Ultrafast energy-dispersive soft-x-ray diffraction in the water window with a laser-driven source.Structural dynamics (Melville, N.Y.) · 2024Article
- A sub-100 nm thickness flat jet for extreme ultraviolet to soft X-ray absorption spectroscopy.Journal of synchrotron radiation · 2024Article
- Toward ultrafast soft x-ray spectroscopy of organic photovoltaic devices.Structural dynamics (Melville, N.Y.) · 2024Article
- 3D-printed sheet jet for stable megahertz liquid sample delivery at X-ray free-electron lasers.IUCrJ · 2023Article
- Thinner than a knife's edge: 3D-printed liquid sheet jet technology for solution phase XFEL experiments.IUCrJ · 2023Article
- Article
- Apparatus for attosecond transient-absorption spectroscopy in the water-window soft-X-ray region.Scientific reports · 2023Article
- HHG at the Carbon K-Edge Directly Driven by SRS Red-Shifted Pulses from an Ytterbium Amplifier.ACS photonics · 2023Article
- Hole Dynamics in Photoexcited Hematite Studied with Femtosecond Oxygen K-edge X-ray Absorption Spectroscopy.The journal of physical chemistry letters · 2022Article
- Delivery of stable ultra-thin liquid sheets in vacuum for biochemical spectroscopy.Frontiers in molecular biosciences · 2022Article
- Temperature measurements of liquid flat jets in vacuum.Structural dynamics (Melville, N.Y.) · 2022Article
- Software for the frontiers of quantum chemistry: An overview of developments in the Q-Chem 5 package.The Journal of chemical physics · 2021Article
- Highly efficient soft x-ray spectrometer for transient absorption spectroscopy with broadband table-top high harmonic sources.Structural dynamics (Melville, N.Y.) · 2021Article
- Ultrafast time-resolved x-ray absorption spectroscopy of ionized urea and its dimer throughStructural dynamics (Melville, N.Y.) · 2021Article
- Shot noise limited soft x-ray absorption spectroscopy in solution at a SASE-FEL using a transmission grating beam splitter.Structural dynamics (Melville, N.Y.) · 2021Article
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Authors and funding
11 authors.
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No grant is acknowledged in the PubMed record.
Abstract
Femtosecond X-ray absorption spectroscopy (XAS) is a powerful method to investigate the dynamical behavior of a system after photoabsorption in real time. So far, the application of this technique has remained limited to large-scale facilities, such as femtosliced synchrotrons and free-electron lasers (FEL). In this work, we demonstrate femtosecond time-resolved soft-X-ray absorption spectroscopy of liquid samples by combining a sub-micrometer-thin flat liquid jet with a high-harmonic tabletop source covering the entire water-window range (284-538 eV). Our work represents the first extension of tabletop XAS to the oxygen edge of a chemical sample in the liquid phase. In the time domain, our measurements resolve the gradual appearance of absorption features below the carbon K-edge of ethanol and methanol during strong-field ionization and trace the valence-shell ionization dynamics of the liquid alcohols with a temporal resolution of ∼30 fs. This technique opens unique opportunities to study molecular dynamics of chemical systems in the liquid phase with elemental, orbital, and site sensitivity.
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