Evidence map›Paper›PMID 32055349›Full record

ArticleChemical science2019

Fluorescence-phosphorescence dual emissive carbon nitride quantum dots show 25% white emission efficiency enabling single-component WLEDs.

Ting Yuan, Fanglong Yuan, Xiaohong Li, Yunchao Li, Louzhen Fan, Shihe Yang

Abstract read
In one paragraph

Article in Chemical science, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.

0numbers the graph read from it
0cells of the map it votes in
18citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

18 citing papers in PubMed.

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  16. Fluorescent Carbon Dots: Fantastic Electroluminescent Materials for Light-Emitting Diodes.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2021
    Review
  17. Article
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

6 authors.

Ting YuanCollege of Chemistry , Beijing Normal University , Beijing , 100875 , China . Email: lzfan@bnu.edu.cn.
Fanglong YuanCollege of Chemistry , Beijing Normal University , Beijing , 100875 , China . Email: lzfan@bnu.edu.cn.
Xiaohong LiCollege of Chemistry , Beijing Normal University , Beijing , 100875 , China . Email: lzfan@bnu.edu.cn.ORCID 0000-0003-2043-1206
Yunchao LiCollege of Chemistry , Beijing Normal University , Beijing , 100875 , China . Email: lzfan@bnu.edu.cn.ORCID 0000-0002-5554-7252
Louzhen FanCollege of Chemistry , Beijing Normal University , Beijing , 100875 , China . Email: lzfan@bnu.edu.cn.ORCID 0000-0002-5245-3234
Shihe YangGuangdong Key Lab of Nano-Micro Material Research , School of Chemical Biology and Biotechnology , Shenzhen Graduate School , Peking University , Shenzhen 518055 , China . Email: chsyang@pku.edu.cn.ORCID 0000-0003-0714-6320

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Developing efficient single-component white light-emitting diodes (WLEDs) is extremely challenging due to the issue of Kasha's rule. Here we report the first demonstration of blue-yellow fluorescence-phosphorescence dual emission from our newly minted single-component white emissive carbon nitride quantum dots (W-CNQDs). The W-CNQDs deliver an overall photoluminescence quantum efficiency of 25%, which is the highest value among white-emitting materials reported to date, based on utilizing both singlet and triplet states. Experimental and theoretical investigations reveal that the carbonyl groups at the rim of the W-CNQDs play a key role in promoting intersystem crossing and inducing intermolecular electronic coupling, affording intensive yellow phosphorescence. Efficient white emission is achieved with a phosphorescence quantum efficiency of 6% under ambient conditions. A WLED is fabricated by integrating W-CNQD phosphors into a UV-LED chip, which shows favorable white light characteristics with CIE coordinates and a CRI of (0.35, 0.39) and 85, respectively, demonstrating good color chromatic stability. This work opens up new opportunities for exploring dual emission mechanisms and designs to facilitate the development of efficient single-component WLEDs.

Identifiers

PMID32055349
PMCPMC6993616

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.