ArticleNature materials2020
Molecular understanding of charge storage and charging dynamics in supercapacitors with MOF electrodes and ionic liquid electrolytes.
Article in Nature materials, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 63 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
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Who cites it
63 citing papers in PubMed.
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- Simulation of Charge Distribution and Microstructure in Semicrystalline Polymeric Ionic-Electronic Conductors Using Classical Simulation at Constant Electrochemical Potential.Journal of chemical theory and computation · 2026Article
- Geometrically Induced Acceleration for Charging Dynamics of Electrical Double-Layers in a Nanopore with Sloped Walls.The journal of physical chemistry. C, Nanomaterials and interfaces · 2026Article
- Biomineralization-mimicking cooperative assembly for tailoring anisotropic hierarchically porous metal-organic frameworks.Chemical science · 2026Article
- Realistic atomic model for charge storage and charging dynamics of amorphous porous carbons.Nature communications · 2026Article
- Density-Potential Functional Theoretic (DPFT) Schemes of Modeling Reactive Solid-Liquid Interfaces.ACS physical chemistry Au · 2025Article
- Sweat Wearable Sensor Based on Confined Pt Nanoparticles in 2D Conductive Metal-Organic Frameworks for Continuous Glucose Monitoring.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Synergistically competitive coordination for tailoring sodium cointercalation potential of graphite.Nature communications · 2025Article
- Revealing Dynamic Ion Transport in Tailorable Carbon Nano-Skyscraper Electrodes.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Molecular Engineering of MXene-Covalent-Triazine Framework Interfaces for Electrochemical Actuators.ACS nano · 2025Article
- Optimizing the Structure and Performances of Cu-MOF@TiNanomaterials (Basel, Switzerland) · 2025Article
- Impact of the Channel Length in Nanoporous Electric Double-Layer Capacitors on the Charge Transport Explored by Metal-Organic Framework Films.ACS physical chemistry Au · 2025Article
- Effect of surface charge on wettability and electrolyte behavior on graphene surfaces using molecular dynamic simulation.Scientific reports · 2025Article
- Highly efficient ionic actuators enabled by sliding ring molecule actuation.Nature communications · 2025Article
- Recent Advances in Probing Electron Delocalization in Conjugated Molecules by Attached Infrared Reporter Groups for Energy Conversion and Storage.ACS applied energy materials · 2025Review
- Balancing the Functionality and Biocompatibility of Materials with a Deep-Learning-Based Inverse Design Framework.Environment & health (Washington, D.C.) · 2024Article
3 more citing papers are in PubMed but not listed here.
Corrections and comments
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Authors and funding
13 authors.
Funding
Abstract
We performed constant-potential molecular dynamics simulations to analyse the double-layer structure and capacitive performance of supercapacitors composed of conductive metal-organic framework (MOF) electrodes and ionic liquids. The molecular modelling clarifies how ions transport and reside inside polarized porous MOFs, and then predicts the corresponding potential-dependent capacitance in characteristic shapes. The transmission line model was adopted to characterize the charging dynamics, which further allowed evaluation of the capacitive performance of this class of supercapacitors at the macroscale from the simulation-obtained data at the nanoscale. These 'computational microscopy' results were supported by macroscopic electrochemical measurements. Such a combined nanoscale-to-macroscale investigation demonstrates the potential of MOF supercapacitors for achieving unprecedentedly high volumetric energy and power densities. It gives molecular insights into preferred structures of MOFs for accomplishing consistent performance with optimal energy-power balance, providing a blueprint for future characterization and design of these new supercapacitor systems.
Identifiers
32015536What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.