ArticleNature communications2020
Charge distribution guided by grain crystallographic orientations in polycrystalline battery materials.
Article in Nature communications, 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 32 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
32 citing papers in PubMed.
- Elucidating ionic-electronic transport in cation-disordered rocksalt cathodes.Chemical science · 2026Review
- Machine Learning Enabled Graph Analysis of Particulate Composites: Application to Solid-State Battery Cathodes.ACS energy letters · 2026Article
- Intrinsic Correlation between Defects, Structure, and Lithium-Ion Transport Kinetics in Epitaxial LiNiACS applied materials & interfaces · 2026Article
- Chemical heterogeneity for battery materials.Nature reviews. Chemistry · 2026Review
- Data-driven deformation correction in X-ray spectro-tomography with implicit neural networks.Patterns (New York, N.Y.) · 2026Article
- Nanostructured niobium-doped nickel-rich multiphase positive electrode active material for high-power lithium-based batteries.Nature nanotechnology · 2026Article
- Unravelling electro-chemo-mechanical interplay in layered oxide cathode degradation in solid-state batteries.Science advances · 2025Article
- Advancing Sodium-Ion Battery Cathodes: A Low-Cost, Eco-Friendly Mechanofusion Route from TiOChemistry of materials : a publication of the American Chemical Society · 2025Article
- Effect of a Two-Step Temperature-Swing Synthesis on Coarse-Grained LiNiOChemistry of materials : a publication of the American Chemical Society · 2025Article
- Thermal processing to modulate surface chemistry and bulk charge distribution in nickel-rich layered lithium positive electrodes.Nature communications · 2025Article
- Article
- Strong Lewis-acid coordinated PEO electrolyte achieves 4.8 V-class all-solid-state batteries over 580 Wh kgNature communications · 2024Article
- Revealing the Chemical and Structural Complexity of Electrochemical Ion Exchange in Layered Oxide Materials.Journal of the American Chemical Society · 2024Article
- Probing Multiscale Dynamics of Energy-Dense Batteries by Operando Imaging.Chem & bio engineering · 2024Review
- Origins and Importance of Intragranular Cracking in Layered Lithium Transition Metal Oxide Cathodes.ACS applied energy materials · 2024Article
- Image registration for in situ X-ray nano-imaging of a composite battery cathode with deformation.Journal of synchrotron radiation · 2024Article
- Kirkendall effect-induced uniform stress distribution stabilizes nickel-rich layered oxide cathodes.Nature communications · 2024Article
- Asynchronous domain dynamics and equilibration in layered oxide battery cathode.Nature communications · 2023Article
- Enabling Electrochemical-Mechanical Robustness of Ultra-High Ni Cathode via Self-Supported Primary-Grain-Alignment Strategy.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Multiscale Imaging Techniques for Real-Time, Noninvasive Diagnosis of Li-Ion Battery Failures.Small science · 2023Article
Corrections and comments
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Authors and funding
16 authors.
Funding
Abstract
Architecting grain crystallographic orientation can modulate charge distribution and chemomechanical properties for enhancing the performance of polycrystalline battery materials. However, probing the interplay between charge distribution, grain crystallographic orientation, and performance remains a daunting challenge. Herein, we elucidate the spatially resolved charge distribution in lithium layered oxides with different grain crystallographic arrangements and establish a model to quantify their charge distributions. While the holistic "surface-to-bulk" charge distribution prevails in polycrystalline particles, the crystallographic orientation-guided redox reaction governs the charge distribution in the local charged nanodomains. Compared to the randomly oriented grains, the radially aligned grains exhibit a lower cell polarization and higher capacity retention upon battery cycling. The radially aligned grains create less tortuous lithium ion pathways, thus improving the charge homogeneity as statistically quantified from over 20 million nanodomains in polycrystalline particles. This study provides an improved understanding of the charge distribution and chemomechanical properties of polycrystalline battery materials.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.