ArticleChemical science2019
Conceptual similarities between zeolites and artificial enzymes.
Article in Chemical science, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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Who cites it
3 citing papers in PubMed, 24 citations in OpenAlex.
- Alkali and Alkaline Earth Metal Oxide-Modified Aluminosilicate and Zeolitic Ceramic Catalysts for Sustainable Biodiesel Production: A Review.ChemPlusChem · 2026Review
- Approaching enzymatic catalysis with zeolites or how to select one reaction mechanism competing with others.Nature communications · 2023Article
- Design and Synthesis of the Active Site Environment in Zeolite Catalysts for Selectively Manipulating Mechanistic Pathways.Journal of the American Chemical Society · 2021Article
Corrections and comments
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Authors and funding
5 authors at 1 institution in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
By using a Diels-Alder (DA) reaction as a base case, we show that a pure silica zeolite acting as an entropy-trapping scaffold can be synthesized with an organic structure directing agent (OSDA) analogue of the transition state (TS) of the DA reaction. A cavity stabilization of the TS is observed with the corresponding decrease in the activation energy of the reaction. A lower enthalpy of activation and a larger decrease in entropy are obtained with the zeolite synthesized with the analogue of the DA TS when compared with other zeolitic structures. Those differences are maintained, while catalytic activity is increased, when active sites are introduced in the zeolite. The catalytic zeolitic system synthesized with the OSDA analogue of the TS shows conceptual similarities with "
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Registered trials
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