ArticleNature communications2019
Enhancement of and interference among higher order multipole transitions in molecules near a plasmonic nanoantenna.
Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. An erratum has been issued. Cited by 6 papers.
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
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Who cites it
6 citing papers in PubMed.
- Freeform Mode-Engineered Metasurfaces.Nano letters · 2026Article
- Interference between multipolar two-photon transitions in quantum emitters near plasmonic nanostructures.Discover nano · 2024Article
- Article
- Asymmetrical Plasmon Distribution in Hybrid AuAg Hollow/Solid Coded Nanotubes.Nanomaterials (Basel, Switzerland) · 2023Article
- Interaction of atomic systems with quantum vacuum beyond electric dipole approximation.Scientific reports · 2020Article
- Interaction and Entanglement of a Pair of Quantum Emitters near a Nanoparticle: Analysis beyond Electric-Dipole Approximation.Entropy (Basel, Switzerland) · 2020Article
Corrections and comments
- Erratum issued
Authors and funding
9 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Spontaneous emission of quantum emitters can be modified by their optical environment, such as a resonant nanoantenna. This impact is usually evaluated under assumption that each molecular transition is dominated only by one multipolar channel, commonly the electric dipole. In this article, we go beyond the electric dipole approximation and take light-matter coupling through higher-order multipoles into account. We investigate a strong enhancement of the magnetic dipole and electric quadrupole emission channels of a molecule adjacent to a plasmonic nanoantenna. Additionally, we introduce a framework to study interference effects between various transition channels in molecules by rigorous quantum-chemical calculations of their multipolar moments and a consecutive investigation of the transition rate upon coupling to a nanoantenna. We predict interference effects between these transition channels, which allow in principle for a full suppression of radiation by exploiting destructive interference, waiving limitations imposed on the emitter's coherence time by spontaneous emission.
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Registered trials
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