ArticleChemistry (Weinheim an der Bergstrasse, Germany)2020
Atomistic Insight Into the Host-Guest Interaction of a Photoresponsive Metal-Organic Framework.
Article in Chemistry (Weinheim an der Bergstrasse, Germany), 2020. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Nanoporous Films with Oriented Arrays of Molecular Motors for Photoswitching the Guest Adsorption and Diffusion.Angewandte Chemie (International ed. in English) · 2023Article
- Modus Operandi of a Pedalo-Type Molecular Switch: Insight from Dynamics and Theoretical Spectroscopy.Molecules (Basel, Switzerland) · 2023Article
- Dynamic network of intermolecular interactions in metal-organic frameworks functionalized by molecular machines.Science advances · 2022Article
- Understanding the Molecular Origin of the Collective Movement in a Diarylethene-based Photo-Responsive Actuator.Chemphyschem : a European journal of chemical physics and physical chemistry · 2021Article
- Atomistic Insight Into the Host-Guest Interaction of a Photoresponsive Metal-Organic Framework.Chemistry (Weinheim an der Bergstrasse, Germany) · 2020Article
Corrections and comments
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Authors and funding
2 authors.
Funding
Abstract
Photoresponsive functional materials have gained increasing attention due to their externally tunable properties. Molecular switches embedded in these materials enable the control of phenomena at the atomic level by light. Metal-organic frameworks (MOFs) provide a versatile platform to immobilize these photoresponsive units within defined molecular environments to optimize the intended functionality. For the application of these photoresponsive MOFs (pho-MOFs), it is crucial to understand the influence of the switching state on the host-guest interaction. Therefore, we present a detailed insight into the impact of molecular switching on the intermolecular interactions. By performing atomistic simulations, we revealed that due to different interactions of the guest molecules with the two isomeric states of an azobenzene-functionalized MOF, both the adsorption sites and the orientation of the molecules within the pores are modulated. By shedding light on the host-guest interaction, our study highlights the unique potential of pho-MOFs to tailor molecular interaction by light.
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