ArticleNature communications2019
Hyperpolarized relaxometry based nuclear T
Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Sensing with discrete time crystals.Nature physics · 2026Article
- Comparing low-field cryogenic nuclear relaxation of hyperpolarized diamond and silicon particles.Scientific reports · 2025Article
- Nanoscale engineering and dynamic stabilization of mesoscopic spin textures.Science advances · 2025Article
- Article
- Relaxation enhancement by microwave irradiation may limit dynamic nuclear polarization.Physical chemistry chemical physics : PCCP · 2024Article
- Optical and electronic spin properties of fluorescent micro- and nanodiamonds upon prolonged ultrahigh-temperature annealing.Journal of vacuum science and technology. B, Nanotechnology & microelectronics : materials, processing, measurement, & phenomena : JVST B · 2023Article
- Advances in Stabilization and Enrichment of Shallow Nitrogen-Vacancy Centers in Diamond for Biosensing and Spin-Polarization Transfer.Biosensors · 2023Review
- Divergent Effects of Laser Irradiation on Ensembles of Nitrogen-Vacancy Centers in Bulk and Nanodiamonds: Implications for Biosensing.Nanoscale research letters · 2022Article
- Optical Dynamic Nuclear Polarization ofMolecules (Basel, Switzerland) · 2022Article
- Long-Lived Ensembles of Shallow NVACS applied materials & interfaces · 2021Article
- Room-temperature hyperpolarization of polycrystalline samples with optically polarized triplet electrons: pentacene or nitrogen-vacancy center in diamond?Magnetic resonance (Gottingen, Germany) · 2021Article
- Signal-enhanced real-time magnetic resonance of enzymatic reactions at millitesla fields.Chemical science · 2020Article
- Carbon-13 dynamic nuclear polarization in diamond via a microwave-free integrated cross effect.Proceedings of the National Academy of Sciences of the United States of America · 2019Article
Corrections and comments
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Authors and funding
17 authors.
Funding
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Abstract
The origins of spin lifetimes in quantum systems is a matter of importance in several areas of quantum information. Spectrally mapping spin relaxation processes provides insight into their origin and motivates methods to mitigate them. In this paper, we map nuclear relaxation in a prototypical system of [Formula: see text] nuclei in diamond coupled to Nitrogen Vacancy (NV) centers over a wide field range (1 mT-7 T). Nuclear hyperpolarization through optically pumped NV electrons allows signal measurement savings exceeding million-fold over conventional methods. Through a systematic study with varying substitutional electron (P1 center) and [Formula: see text] concentrations, we identify the operational relaxation channels for the nuclei at different fields as well as the dominant role played by [Formula: see text] coupling to the interacting P1 electronic spin bath. These results motivate quantum control techniques for dissipation engineering to boost spin lifetimes in diamond, with applications including engineered quantum memories and hyperpolarized [Formula: see text] imaging.
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