ArticleScientific reports2019
Investigating the Integrity of Graphene towards the Electrochemical Hydrogen Evolution Reaction (HER).
Article in Scientific reports, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
11 citing papers in PubMed.
- Laser Synthesis of Platinum Single-Atom Catalysts for Hydrogen Evolution Reaction.Nanomaterials (Basel, Switzerland) · 2025Article
- Laser-Induced Vertical Graphene Nanosheets for Electrocatalytic Hydrogen Evolution.ACS applied nano materials · 2024Article
- Recent Advances in Carbon-Based Electrodes for Energy Storage and Conversion.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Review
- Materials Screening by the DescriptorACS catalysis · 2023Review
- 2D-Hexagonal Boron Nitride Screen-Printed Bulk-Modified Electrochemical Platforms Explored towards Oxygen Reduction Reactions.Sensors (Basel, Switzerland) · 2022Article
- Bidirectional Hydrogen Electrocatalysis on Epitaxial Graphene.ACS omega · 2022Article
- Laser solid-phase synthesis of single-atom catalysts.Light, science & applications · 2021Article
- Investigation of polymer-derived Si-(B)-C-N ceramic/reduced graphene oxide composite systems as active catalysts towards the hydrogen evolution reaction.Scientific reports · 2020Article
- Electrochemical properties of vertically aligned graphenes: tailoring heterogeneous electron transfer through manipulation of the carbon microstructure.Nanoscale advances · 2020Article
- Graphene Oxide Bulk-Modified Screen-Printed Electrodes Provide Beneficial Electroanalytical Sensing Capabilities.Biosensors · 2020Article
- Tailoring the electrochemical properties of 2D-hBNNanoscale advances · 2020Article
Corrections and comments
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Authors and funding
3 authors.
Funding
Abstract
Mono-, few-, and multilayer graphene is explored towards the electrochemical Hydrogen Evolution Reaction (HER). Careful physicochemical characterisation is undertaken during electrochemical perturbation revealing that the integrity of graphene is structurally compromised. Electrochemical perturbation, in the form of electrochemical potential scanning (linear sweep voltammetry), as induced when exploring the HER using monolayer graphene, creates defects upon the basal plane surface that increases the coverage of edge plane sites/defects resulting in an increase in the electrochemical reversibility of the HER process. This process of improved HER performance occurs up to a threshold, where substantial break-up of the basal sheet occurs, after which the electrochemical response decreases; this is due to the destruction of the sheet integrity and lack of electrical conductive pathways. Importantly, the severity of these changes is structurally dependent on the graphene variant utilised. This work indicates that multilayer graphene has more potential as an electrochemical platform for the HER, rather than that of mono- and few-layer graphene. There is huge potential for this knowledge to be usefully exploited within the energy sector and beyond.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.