ArticleNature communications2019
Core-level nonlinear spectroscopy triggered by stochastic X-ray pulses.
Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Single-shot hard X-ray spectrometer with uniform spatial and spectral response.Journal of synchrotron radiation · 2026Article
- Article
- STEP: extraction of underlying physics with robust machine learning.Royal Society open science · 2024Article
- Experimental capabilities for liquid jet samples at sub-MHz rates at the FXE Instrument at European XFEL.Journal of synchrotron radiation · 2023Article
- The case for data science in experimental chemistry: examples and recommendations.Nature reviews. Chemistry · 2022Review
- Transient measurement of phononic states with covariance-based stochastic spectroscopy.Light, science & applications · 2022Article
- Spectral monitoring at SwissFEL using a high-resolution on-line hard X-ray single-shot spectrometer.Journal of synchrotron radiation · 2021Article
- Unveiling the spatial distribution of molecular coherences at conical intersections by covariance X-ray diffraction signals.Proceedings of the National Academy of Sciences of the United States of America · 2021Article
- X-ray-Based Techniques to Study the Nano-Bio Interface.ACS nano · 2021Article
- XABOOM: An X-ray Absorption Benchmark of Organic Molecules Based on Carbon, Nitrogen, and Oxygen 1s → π* Transitions.Journal of chemical theory and computation · 2021Article
- Resonant X-ray emission spectroscopy from broadband stochastic pulses at an X-ray free electron laser.Communications chemistry · 2021Article
Corrections and comments
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Authors and funding
18 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Stochastic processes are highly relevant in research fields as different as neuroscience, economy, ecology, chemistry, and fundamental physics. However, due to their intrinsic unpredictability, stochastic mechanisms are very challenging for any kind of investigations and practical applications. Here we report the deliberate use of stochastic X-ray pulses in two-dimensional spectroscopy to the simultaneous mapping of unoccupied and occupied electronic states of atoms in a regime where the opacity and transparency properties of matter are subject to the incident intensity and photon energy. A readily transferable matrix formalism is presented to extract the electronic states from a dataset measured with the monitored input from a stochastic excitation source. The presented formalism enables investigations of the response of the electronic structure to irradiation with intense X-ray pulses while the time structure of the incident pulses is preserved.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.