Evidence map›Paper›PMID 31601795›Full record

ArticleNature communications2019

Interplay between structural hierarchy and exciton diffusion in artificial light harvesting.

Björn Kriete, Julian Lüttig, Tenzin Kunsel, Pavel Malý, Thomas L C Jansen, Jasper Knoester, Tobias Brixner, Maxim S Pshenichnikov

Abstract read
In one paragraph

Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 20 papers.

0numbers the graph read from it
0cells of the map it votes in
20citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

20 citing papers in PubMed.

  1. Article
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  6. Article
  7. Article
  8. Watching Molecular Nanotubes Self-Assemble in Real Time.Journal of the American Chemical Society · 2023
    Article
  9. Article
  10. Article
  11. Article
  12. Article
  13. Article
  14. Article
  15. Article
  16. 2D Electronic Spectroscopic Techniques for Quantum Technology Applications.The journal of physical chemistry. C, Nanomaterials and interfaces · 2021
    Review
  17. Article
  18. Article
  19. Article
  20. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Björn KrieteUniversity of Groningen, Zernike Institute for Advanced Materials, Nijenborgh 4, 9747 AG, Groningen, The Netherlands.
Julian LüttigInstitut für Physikalische und Theoretische Chemie, Universität Würzburg, Am Hubland, 97074, Würzburg, Germany.
Tenzin KunselUniversity of Groningen, Zernike Institute for Advanced Materials, Nijenborgh 4, 9747 AG, Groningen, The Netherlands.ORCID http://orcid.org/0000-0002-6103-6635
Pavel MalýInstitut für Physikalische und Theoretische Chemie, Universität Würzburg, Am Hubland, 97074, Würzburg, Germany.
Thomas L C JansenUniversity of Groningen, Zernike Institute for Advanced Materials, Nijenborgh 4, 9747 AG, Groningen, The Netherlands.ORCID http://orcid.org/0000-0001-6066-6080
Jasper KnoesterUniversity of Groningen, Zernike Institute for Advanced Materials, Nijenborgh 4, 9747 AG, Groningen, The Netherlands.
Tobias BrixnerInstitut für Physikalische und Theoretische Chemie, Universität Würzburg, Am Hubland, 97074, Würzburg, Germany.ORCID http://orcid.org/0000-0002-6529-704X
Maxim S PshenichnikovUniversity of Groningen, Zernike Institute for Advanced Materials, Nijenborgh 4, 9747 AG, Groningen, The Netherlands. M.S.Pchenitchnikov@rug.nl.

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Unraveling the nature of energy transport in multi-chromophoric photosynthetic complexes is essential to extract valuable design blueprints for light-harvesting applications. Long-range exciton transport in such systems is facilitated by a combination of delocalized excitation wavefunctions (excitons) and exciton diffusion. The unambiguous identification of the exciton transport is intrinsically challenging due to the system's sheer complexity. Here we address this challenge by employing a spectroscopic lab-on-a-chip approach: ultrafast coherent two-dimensional spectroscopy and microfluidics working in tandem with theoretical modeling. We show that at low excitation fluences, the outer layer acts as an exciton antenna supplying excitons to the inner tube, while under high excitation fluences the former converts its functionality into an exciton annihilator which depletes the exciton population prior to any exciton transfer. Our findings shed light on the excitonic trajectories across different sub-units of a multi-layered artificial light-harvesting complex and underpin their great potential for directional excitation energy transport.

Identifiers

PMID31601795
PMCPMC6787233

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.