ArticleScience advances2019
Size-dependent thermodynamic structural selection in colloidal crystallization.
Article in Science advances, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Spatially programmed polymorphic crystallization via microenvironment design.Science advances · 2026Article
- Self-assembly pathways towards floppy colloidal square lattices.Nature communications · 2025Article
- Article
- Two-step crystallization and solid-solid transitions in binary colloidal mixtures.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
- Hydrodynamic and frictional modulation of deformations in switchable colloidal crystallites.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
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Authors and funding
6 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Nucleation and growth of crystalline phases play an important role in a variety of physical phenomena, ranging from freezing of liquids to assembly of colloidal particles. Understanding these processes in the context of colloidal crystallization is of great importance for predicting and controlling the structures produced. In many systems, crystallites that nucleate have structures differing from those expected from bulk equilibrium thermodynamic considerations, and this is often attributed to kinetic effects. In this work, we consider the self-assembly of a binary mixture of colloids in two dimensions, which exhibits a structural transformation from a non-close-packed to a close-packed lattice during crystal growth. We show that this transformation is thermodynamically driven, resulting from size dependence of the relative free energy between the two structures. We demonstrate that structural selection can be entirely thermodynamic, in contrast to previously considered effects involving growth kinetics or interaction with the surrounding fluid phase.
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Registered trials
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