ArticleACS central science2019
A Molecular Coordination Template Strategy for Designing Selective Porous Aromatic Framework Materials for Uranyl Capture.
Article in ACS central science, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed, 121 citations in OpenAlex.
- Ultrafast, High-Capacity Uranium Harvesting From Seawater via a Hierarchically Porous Polymer Electrode.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Synergistic Adsorption and Fluorescence in Porous Aromatic Frameworks for Highly Sensitive Detection of Radioactive Uranium.Molecules (Basel, Switzerland) · 2025Article
- Ultra-selective uranium separation by in-situ formation of π-f conjugated 2D uranium-organic framework.Nature communications · 2024Article
- Self-Standing Porous Aromatic Framework Electrodes for Efficient Electrochemical Uranium Extraction.ACS central science · 2023Article
- Article
- Arrangement of Indocyanine Green in a 1.5-Nanometer Channel to Achieve High-Efficiency Imaging of the Intestinal Lymphatic System.Molecules (Basel, Switzerland) · 2022Article
- Highly Efficient Electrocatalytic Uranium Extraction from Seawater over an Amidoxime-Functionalized In-N-C Catalyst.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2022Article
- Article
- A Facile and Highly Efficient Approach to Obtain a Fluorescent Chromogenic Porous Organic Polymer for Lymphatic Targeting Imaging.Molecules (Basel, Switzerland) · 2022Article
- Ionic Porous Aromatic Framework as a Self-Degraded Template for the Synthesis of a Magnetic γ-FeMolecules (Basel, Switzerland) · 2021Article
- Nanospace Decoration with Uranyl-Specific "Hooks" for Selective Uranium Extraction from Seawater with Ultrahigh Enrichment Index.ACS central science · 2021Article
- Molecularly Imprinted Porous Aromatic Frameworks for Molecular Recognition.ACS central science · 2020Review
- Hydroxyl porous aromatic frameworks for efficient adsorption of organic micropollutants in water.RSC advances · 2020Article
- Constructing amidoxime-modified porous adsorbents with open architecture for cost-effective and efficient uranium extraction.Chemical science · 2020Article
- Mystical Material Might Help Solve Global Energy Problems.ACS central science · 2019Article
Corrections and comments
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Authors and funding
12 authors at 4 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Uranium capture from seawater could solve increasing energy demand and enable a much needed relaxing from fossil fuels. Low concentration (∼3 ppb), competing cations (especially vanadium) and pH-dependent speciation prohibit highly efficient uranium uptake. Despite intensive research, selective extraction of uranyl ions over vanadyl units remains a tremendous challenge. Here, we adopted a molecular coordination template strategy to design a uranyl-specific bis-salicylaldoxime entity and decorated it into a highly porous aromatic framework (PAF-1) by programmable assembly. The superstructure (MISS-PAF-1) gives a strong affinity that removes 99.97% of uranium in 120 min. Notably, it binds to the uranyl ion at least 100 times more selectively than 14 different cations tested, including the vanadyl ion, in simulated seawater at ambient pH. Real seawater samples collected from the Bohai Sea achieve 5.79 mg g
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.