ArticleNano letters2019
Photon Correlation Spectroscopy of Luminescent Quantum Defects in Carbon Nanotubes.
Article in Nano letters, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
What it found
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Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
7 citing papers in PubMed.
- Deterministic Formation of Single Organic Color Centers in Single-Walled Carbon Nanotubes.Nano letters · 2025Article
- Chemical Patterning on Nanocarbons: Functionality Typewriting.Molecules (Basel, Switzerland) · 2023Review
- Investigating Molecular Exciton Polaritons UsingThe journal of physical chemistry letters · 2023Article
- Over Two-Fold Photoluminescence Enhancement from Single-Walled Carbon Nanotubes Induced by Oxygen Doping.Nanomaterials (Basel, Switzerland) · 2023Article
- Signatures of Chemical Dopants in Simulated Resonance Raman Spectroscopy of Carbon Nanotubes.The journal of physical chemistry letters · 2023Article
- Synthetic control over the binding configuration of luminescent spNature communications · 2021Article
- Interaction of Luminescent Defects in Carbon Nanotubes with Covalently Attached Stable Organic Radicals.ACS nano · 2021Article
Corrections and comments
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Defect-decorated single-wall carbon nanotubes have shown rapid growing potential for imaging, sensing, and the development of room-temperature single-photon sources. The key to the highly nonclassical emission statistics is the discrete energy spectrum of defect-localized excitons. However, variations in defect configurations give rise to distinct spectral bands that may compromise single-photon efficiency and purity in practical devices, and experimentally it has been challenging to study the exciton population distribution among the various defect-specific states. Here, we performed photon correlation spectroscopy on hexyl-decorated single-wall carbon nanotubes to unravel the dynamics and competition between neutral and charged exciton populations. With autocorrelation measurements at the single-tube level, we prove the nonclassical photon emission statistics of defect-specific exciton and trion photoluminescence and identify their mutual exclusiveness in photoemissive events with cross-correlation spectroscopy. Moreover, our study reveals the presence of a dark state with population-shelving time scales between 10 and 100 ns. These new insights will guide further development of chemically tailored carbon nanotube states for quantum photonics applications.
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