Evidence map›Paper›PMID 31448600›Full record

ArticleJournal of the American Chemical Society2019

Spatiotemporal Quantification of Lithium both in Electrode and in Electrolyte with Atomic Precision via Operando Neutron Absorption.

Peter-Paul R M L Harks, Tomas W Verhallen, Chandramohan George, Jan Karel van den Biesen, Qian Liu, Marnix Wagemaker, Fokko M Mulder

Open access · hybridAbstract read
In one paragraph

Article in Journal of the American Chemical Society, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
1.0field-weighted citation impact, top 24% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed, 18 citations in OpenAlex.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

7 authors at 2 institutions in 2 countries.

Peter-Paul R M L HarksMaterials for Energy Conversion and Storage (MECS), Department of Chemical Engineering , Delft University of Technology , P.O. Box 5045, 2600 GA Delft , The Netherlands.
Tomas W VerhallenDepartment of Radiation Science and Technology , Delft University of Technology , Mekelweg 15 , 2629 JB , Delft , The Netherlands.ORCID http://orcid.org/0000-0002-8473-4321
Chandramohan GeorgeDepartment of Radiation Science and Technology , Delft University of Technology , Mekelweg 15 , 2629 JB , Delft , The Netherlands.ORCID http://orcid.org/0000-0003-2906-6399
Jan Karel van den BiesenDepartment of Radiation Science and Technology , Delft University of Technology , Mekelweg 15 , 2629 JB , Delft , The Netherlands.
Qian LiuDepartment of Radiation Science and Technology , Delft University of Technology , Mekelweg 15 , 2629 JB , Delft , The Netherlands.
Marnix WagemakerDepartment of Radiation Science and Technology , Delft University of Technology , Mekelweg 15 , 2629 JB , Delft , The Netherlands.ORCID http://orcid.org/0000-0003-3851-1044
Fokko M MulderMaterials for Energy Conversion and Storage (MECS), Department of Chemical Engineering , Delft University of Technology , P.O. Box 5045, 2600 GA Delft , The Netherlands.ORCID http://orcid.org/0000-0003-0526-7081
Delft University of Technology · NLDyson (United Kingdom) · GB

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

The commercial uptake of lithium-sulfur (Li-S) batteries is undermined by their rapid performance decay and short cycle life. These problems originate from the dissolution of lithium polysulfide in liquid electrolytes, causing charge and active material to shuttle between electrodes. The dynamics of intractable polysulfide migration at different length scales often tend to escape the probing ability of many analytical techniques. Spatial and temporal visualization of Li in Li-S electrodes and direct mechanistic understanding of how polysulfides are regulated across Li-S batteries starting from current collector and active layer coating to electrode-electrolyte interface are still lacking. To address this we employ neutron depth profiling across Li-S electrodes using the naturally occurring isotope,

Identifiers

PMID31448600
PMCPMC6876927
OpenAlexW2969779357

What OpenQuestion holds

Textmetadata
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.