ArticleNature communications2019
Coherent anti-Stokes Raman spectroscopy of single and multi-layer graphene.
Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 13 papers.
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Who cites it
13 citing papers in PubMed.
- Phonon-Modulated Kerr Nonlinearity in Ultrathin 2Small science · 2026Article
- Coherent Vibrational Anti-Stokes Raman Spectroscopy Assisted by Pulse Shaping.Molecules (Basel, Switzerland) · 2025Review
- Coherent Anti-Stokes Hyper-Raman Spectroscopy.Nature communications · 2025Article
- Current Applications of Raman Spectroscopy in Intraoperative Neurosurgery.Biomedicines · 2024Review
- Numerical study of transient absorption saturation in single-layer graphene for optical nanoscopy applications.Scientific reports · 2024Article
- Imaging and controlling coherent phonon wave packets in single graphene nanoribbons.Nature communications · 2023Article
- Full-Quantum Treatment of Molecular Systems Confirms Novel Supracence Photonic Properties.International journal of molecular sciences · 2023Article
- Picosecond energy transfer in a transition metal dichalcogenide-graphene heterostructure revealed by transient Raman spectroscopy.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Excited-State Energy Surfaces in Molecules Revealed by Impulsive Stimulated Raman Excitation Profiles.The journal of physical chemistry letters · 2021Article
- Non-linear self-driven spectral tuning of Extreme Ultraviolet Femtosecond Pulses in monoatomic materials.Light, science & applications · 2021Article
- Characterization of thymine microcrystals by CARS and SHG microscopy.Scientific reports · 2020Article
- Accessing Excited State Molecular Vibrations by Femtosecond Stimulated Raman Spectroscopy.The journal of physical chemistry letters · 2020Article
- Recognition of Spatial Distribution of CNT and Graphene in Hybrid Structure by Mapping with Coherent Anti-Stokes Raman Microscopy.Nanoscale research letters · 2020Article
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Authors and funding
8 authors.
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Abstract
Spontaneous Raman spectroscopy is a powerful characterization tool for graphene research. Its extension to the coherent regime, despite the large nonlinear third-order susceptibility of graphene, has so far proven challenging. Due to its gapless nature, several interfering electronic and phononic transitions concur to generate its optical response, preventing to retrieve spectral profiles analogous to those of spontaneous Raman. Here we report stimulated Raman spectroscopy of the G-phonon in single and multi-layer graphene, through coherent anti-Stokes Raman Scattering. The nonlinear signal is dominated by a vibrationally non-resonant background, obscuring the Raman lineshape. We demonstrate that the vibrationally resonant coherent anti-Stokes Raman Scattering peak can be measured by reducing the temporal overlap of the laser excitation pulses, suppressing the vibrationally non-resonant background. We model the spectra, taking into account the electronically resonant nature of both. We show how coherent anti-Stokes Raman Scattering can be used for graphene imaging with vibrational sensitivity.
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