ArticleNature communications2019
Visualization and design of the functional group distribution during statistical copolymerization.
Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
What it found
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Who cites it
7 citing papers in PubMed.
- Gradient Copolymers: A Complex Comonomer Incorporation Reality behind the Perfect Ideal.ACS polymers Au · 2026Review
- The successful impossible radical ring-opening copolymerization of thionolactones and methacrylates via an auxiliary third comonomer.Nature communications · 2025Article
- Machine-Learning Approach to Identify Organic Functional Groups from FT-IR and NMR Spectral Data.ACS omega · 2025Article
- Photomediated Cationic Ring-Opening Polymerization of Cyclosiloxanes with Temporal Control.JACS Au · 2024Article
- Molecular Pathways for Polymer Degradation during Conventional Processing, Additive Manufacturing, and Mechanical Recycling.Molecules (Basel, Switzerland) · 2023Review
- Computational prediction of the molecular configuration of three-dimensional network polymers.Nature materials · 2021Article
- Copolymer chain formation of 2-oxazolines byRSC advances · 2021Article
Corrections and comments
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Even though functional copolymers with a low percentage of functional comonomer units (up to 20 mol%) are widely used, for instance for the development of polymer therapeutics and hydrogels, insights in the functional group distribution over the actual chains are lacking and the average composition is conventionally used to describe the functionalization degree. Here we report the visualization of the monomer distribution over the different polymer chains by a synergetic combination of experimental and theoretical analysis aiming at the construction of functionality-chain length distributions (FUNC-CLDs). A successful design of the chemical structure of the comonomer pair, the initial functional comonomer amount (13 mol%), and the temperature (100 °C) is performed to tune the FUNC-CLD of copoly(2-oxazoline)s toward high functionalization degree for both low (100) and high (400) target degrees of polymerization. The proposed research strategy is generic and extendable to a broad range of copolymerization chemistries, including reversible deactivation radical polymerization.
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Registered trials
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