ArticleProceedings of the National Academy of Sciences of the United States of America2019
Direct observation of 2-dimensional ices on different surfaces near room temperature without confinement.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- How surface charges affect interdroplet freezing.Proceedings of the National Academy of Sciences of the United States of America · 2025Article
- Two-dimensional bilayer ice in coexistence with three-dimensional ice without confinement.Nature communications · 2024Article
- Temperature-pressure phase diagram of confined monolayer water/ice at first-principles accuracy with a machine-learning force field.Nature communications · 2023Article
- Ice friction at the nanoscale.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Two-dimensional monolayer salt nanostructures can spontaneously aggregate rather than dissolve in dilute aqueous solutions.Nature communications · 2021Article
- Temperature-dependent kinetic pathways of heterogeneous ice nucleation competing between classical and non-classical nucleation.Nature communications · 2021Article
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Water-solid interfaces play important roles in a wide range of fields, including atmospheric science, geochemistry, electrochemistry, and food science. Herein, we report simulation evidence of 2-dimensional (2D) ice formation on various surfaces and the dependence of the 2D crystalline structure on the hydrophobicity and morphology of the underlying surface. Contrary to the prevailing view that nanoscale confinement is necessary for the 2D liquid-to-bilayer ice transition, we find that the liquid-to-bilayer hexagonal ice (BHI) transition can occur either on a model smooth surface or on model fcc-crystal surfaces with indices of (100), (110), and (111) near room temperature. We identify a critical parameter that characterizes the water-surface interaction, above which the BHI can form on the surface. This critical parameter increases as the temperature increases. Even at temperatures above the freezing temperature of bulk ice (
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