ArticleChemical science2019
Metal-ligand covalency enables room temperature molecular qubit candidates.
Article in Chemical science, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 27 papers.
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Who cites it
27 citing papers in PubMed.
- Molecular Qubits for Anion Sensing by Tuning Electron Spin Relaxation via Axial Ligand Field.Angewandte Chemie (International ed. in English) · 2026Article
- Quantum coherence enhancement through control of metal-ligand covalency: modulating spin-orbit coupling in isostructural molecular qubits.Chemical science · 2026Article
- Enlarging Quantum Coherence of Vanadyl Spin Qubits in Zirconium Porphyrinic MOFs.Inorganic chemistry · 2026Article
- Orientationally Resolved Electron-Spin Relaxation and Coherence in Fullerene-Encapsulated Rare-Earth Dimers with a Single-Electron Metal-Metal Bond.Journal of the American Chemical Society · 2026Article
- Bridging Vibrations and Spins: Mode-Resolved Spin-Phonon Coupling Revealed through THz EPR/Magnetic IR Simulation.The journal of physical chemistry. A · 2026Article
- Novel amide-based macrocyclic Co(ii) complexes: correlating structural, computational, and biological properties through DFT and docking.RSC advances · 2026Article
- A Multireference Picture of Electronic Excited States in Vanadyl and Copper Tetraphenyl Porphyrin Molecular Qubits.The journal of physical chemistry. A · 2025Article
- Spin Coherence and Electron Spin Distribution of a Silver(II)Inorganic chemistry · 2025Article
- Slow Electron Spin Relaxation at Ambient Temperatures with Copper Coordinated by a Rigid Macrocyclic Ligand.Journal of the American Chemical Society · 2025Article
- The role of electronic excited states in the spin-lattice relaxation of spin-1/2 molecules.Science advances · 2025Article
- A Spectrochemical Series for Electron Spin Relaxation.Journal of the American Chemical Society · 2025Article
- Phononic modulation of spin-lattice relaxation in molecular qubit frameworks.Nature communications · 2024Article
- Spectroscopic Signatures of Phonon Character in Molecular Electron Spin Relaxation.ACS central science · 2024Article
- Low temperature decoherence dynamics in molecular spin systems using the Lindblad master equation.Chemical science · 2024Article
- Stable organic radical qubits and their applications in quantum information science.Innovation (Cambridge (Mass.)) · 2024Review
- Ligand Effects on the Spin Relaxation Dynamics and Coherent Manipulation of Organometallic La(II) Potential QuJournal of the American Chemical Society · 2024Article
- Determining the key vibrations for spin relaxation in ruffled Cu(ii) porphyrinsChemical science · 2024Article
- Synthesis, structural characterization, antioxidant, cytotoxic activities and docking studies of schiff base Cu(II) complexes.Heliyon · 2023Article
- A Review of the Current State of Magnetic Force Microscopy to Unravel the Magnetic Properties of Nanomaterials Applied in Biological Systems and Future Directions for Quantum Technologies.Nanomaterials (Basel, Switzerland) · 2023Review
- Two-Electron Mixed Valency in a Heterotrimetallic Nickel-Vanadium-Nickel Complex.Inorganic chemistry · 2023Article
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Authors and funding
6 authors.
Funding
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Abstract
Harnessing synthetic chemistry to design electronic spin-based qubits, the smallest unit of a quantum information system, enables us to probe fundamental questions regarding spin relaxation dynamics. We sought to probe the influence of metal-ligand covalency on spin-lattice relaxation, which comprises the upper limit of coherence time. Specifically, we studied the impact of the first coordination sphere on spin-lattice relaxation through a series of four molecules featuring V-S, V-Se, Cu-S, and Cu-Se bonds, the Ph
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