Evidence map›Paper›PMID 31366945›Full record

ArticleNature communications2019

Many-body simulation of two-dimensional electronic spectroscopy of excitons and trions in monolayer transition metal dichalcogenides.

Roel Tempelaar, Timothy C Berkelbach

Abstract read
In one paragraph

Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. The Low-Temperature Photocurrent Spectrum of Monolayer MoSeNanomaterials (Basel, Switzerland) · 2022
    Article
  5. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

2 authors.

Roel TempelaarDepartment of Chemistry, Columbia University, New York, NY, 10027, USA. r.tempelaar@gmail.com.ORCID http://orcid.org/0000-0003-0786-7304
Timothy C BerkelbachDepartment of Chemistry, Columbia University, New York, NY, 10027, USA. tim.berkelbach@gmail.com.

Funding

United States Department of Defense | United States Air Force | AFMC | Air Force Office of Scientific Research (AF Office of Scientific Research) FA9550-18-1-0058
6 · The paper itself

Abstract

Indications of coherently interacting excitons and trions in doped transition metal dichalcogenides have been measured as quantum beats in two-dimensional electronic spectroscopy, but the microscopic principles underlying the optical signals of exciton-trion coherence remain to be clarified. Here we present calculations of two-dimensional spectra of such monolayers based on a microscopic many-body formalism. We use a parameterized band structure and a static model dielectric function, although a full ab initio implementation of our formalism is possible in principle. Our simulated spectra are in excellent agreement with experiments, including the quantum beats, while revealing the interplay between excitons and trions in molybdenum- and tungsten-based transition metal dichalcogenides. Quantum beats are confirmed to unambiguously reflect the exciton-trion coherence time in molybdenum compounds, but are shown to provide a lower bound to the coherence time for tungsten analogues due to a destructive interference from coexisting singlet and triplet trions.

Identifiers

PMID31366945
PMCPMC6668418

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.