ArticleNature chemistry2019
Super-resolution imaging of non-fluorescent reactions via competition.
Article in Nature chemistry, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 32 papers.
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Who cites it
32 citing papers in PubMed.
- High-resolution studies of photo(electro)catalysts by electrochemical scanning probe microscopy.Chemical science · 2026Review
- Single-particle catalytic monitoring of interfacial charge dynamics during light-driven CdS shell growth on Au nanocubes.Nature communications · 2026Article
- Optical nanoscopy of spatiotemporal metal stripping cooperativity at single-ion and subparticle resolution.Nature materials · 2026Article
- Designing Microbe-Semiconductor Interfaces for Semibiological Photosynthesis.Chemical reviews · 2026Review
- Nanoscale Chemical Imaging of Basic Sites Distribution on Catalytically Active Mg-Al Mixed Oxide Particles.Chemical & biomedical imaging · 2025Article
- A surface chemistry perspective on SERS: revisiting the basics to push the field forward.Chemical Society reviews · 2025Review
- Single-Molecule Fluorescence Imaging of Energy-Related Catalytic Reactions.Chemical & biomedical imaging · 2025Review
- Fluorogenic Linkage Integration for Nonfluorescent Transformations (FLINT).Chemical & biomedical imaging · 2025Article
- Guided electrocatalyst design through in-situ techniques and data mining approaches.Nano convergence · 2025Review
- Probing Multiscale Dynamics of Energy-Dense Batteries by Operando Imaging.Chem & bio engineering · 2024Review
- Surface photovoltage microscopy for mapping charge separation on photocatalyst particles.Nature protocols · 2024Review
- Revealing operando surface defect-dependent electrocatalytic performance of Pt at the subparticle level.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Real-Time Tracking of Vesicles in Living Cells Reveals That Tau-Hyperphosphorylation Suppresses Unidirectional Transport by Motor Proteins.Chemical & biomedical imaging · 2024Article
- Correlating activities and defects in (photo)electrocatalysts using in-situ multi-modal microscopic imaging.Nature communications · 2024Article
- Performance evaluation and multidisciplinary analysis of catalytic fixation reactions by material-microbe hybrids.Nature catalysis · 2024Article
- Nanoscale Luminescence Imaging/Detection of Single Particles: State-of-the-Art and Future Prospects.ACS measurement science au · 2024Review
- Molecular-scale Insights into Cooperativity Switching ofACS central science · 2024Article
- Article
- Getting the Most Out of Fluorogenic Probes: Challenges and Opportunities in Using Single-Molecule Fluorescence to Image Electro- and Photocatalysis.Chemical & biomedical imaging · 2023Review
- Label-Free Imaging of Catalytic HACS nano · 2023Article
Corrections and comments
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Super-resolved fluorescence microscopy techniques have enabled substantial advances in the chemical and biological sciences. However, they can only interrogate entities that fluoresce, and most chemical or biological processes do not involve fluorescent species. Here we report a competition-enabled imaging technique with super-resolution (COMPEITS) that enables quantitative super-resolution imaging of non-fluorescent processes. It is based on the incorporation of competition into a single-molecule fluorescence-detection scheme. We demonstrate COMPEITS by investigating a photoelectrocatalytic reaction; we map, with nanometre precision, a non-fluorescent surface reaction that is important for water decontamination on single photocatalyst particles. The subparticle-level quantitative information of reactant adsorption affinities unambiguously decouples size- and shape-scaling laws on specific particle facets and uncovers a surprising biphasic shape dependence, leading to catalyst design principles for optimal reactant adsorption efficacy. With its ability to provide spatially resolved information on the behaviours of unlabelled, non-fluorescent entities under operando conditions, COMPEITS could interrogate a variety of surface processes in fields ranging from heterogeneous catalysis and materials engineering to nanotechnology and energy sciences.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.