ArticleScience advances2019
A high-spin ground-state donor-acceptor conjugated polymer.
Article in Science advances, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 20 papers.
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Who cites it
20 citing papers in PubMed.
- Single-atom photocatalyst for click reaction.Nature communications · 2026Article
- Modular Donor-Acceptor Diradicaloids Based on an Electron Deficient N-Heteroacene Acceptor.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Role of π-Spacers and Acceptors in Regulating the Photophysical Properties of BTPA Donor-Based Dyes: First-Principles Approach.The journal of physical chemistry. A · 2025Article
- Solid-State Quantum Coherence From a High-Spin Donor-Acceptor Conjugated Polymer.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Long-Range Resonant Charge Transport through Open-Shell Donor-Acceptor Macromolecules.Journal of the American Chemical Society · 2025Article
- Stable Open-Shell Conjugated Terpolymer with Extended NIR Absorption for Organic Photodetectors Detecting Beyond 1000 nm.ACS applied materials & interfaces · 2025Article
- Halogenated-edge polymeric semiconductor for efficient spin transport.Nature communications · 2024Article
- Extended shortwave infrared absorbing antiaromatic fluorenium-indolizine chromophores.Chemical science · 2024Article
- A high-spinRSC advances · 2024Article
- Designing Thiadiazoloquinoxaline-Based Conjugated Polymers for Efficient Organic Photovoltaics: A DFT/TDDFT Study.Molecules (Basel, Switzerland) · 2024Article
- Electronic properties and optical spectra of donor-acceptor conjugated organic polymers.Scientific reports · 2023Article
- Ultrasensitive Room Temperature Infrared Photodetection Using a Narrow Bandgap Conjugated Polymer.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
- Enhanced sub-1 eV detection in organic photodetectors through tuning polymer energetics and microstructure.Science advances · 2023Article
- Organic radicals stabilization above 300 °C in Eu-based coordination polymers for solar steam generation.Nature communications · 2022Article
- High-mobility semiconducting polymers with different spin ground states.Nature communications · 2022Article
- Red edge effect and chromoselective photocatalysis with amorphous covalent triazine-based frameworks.Nature communications · 2022Article
- Evolution of the electronic structure in open-shell donor-acceptor organic semiconductors.Nature communications · 2021Article
- Broadband infrared photodetection using a narrow bandgap conjugated polymer.Science advances · 2021Article
- Donor-Acceptor Conjugated Macrocycles with Polyradical Character and Global Aromaticity.iScience · 2020Article
- Three-Dimensional Visualization for Early-Stage Evolution of Polymer Aging.ACS central science · 2020Article
Corrections and comments
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Authors and funding
13 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Interest in high-spin organic materials is driven by opportunities to enable far-reaching fundamental science and develop technologies that integrate light element spin, magnetic, and quantum functionalities. Although extensively studied, the intrinsic instability of these materials complicates synthesis and precludes an understanding of how fundamental properties associated with the nature of the chemical bond and electron pairing in organic materials systems manifest in practical applications. Here, we demonstrate a conjugated polymer semiconductor, based on alternating cyclopentadithiophene and thiadiazoloquinoxaline units, that is a ground-state triplet in its neutral form. Electron paramagnetic resonance and magnetic susceptibility measurements are consistent with a high-to-low spin energy gap of 9.30 × 10
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.