ArticleNature communications2019
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking.
Article in Nature communications, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 17 papers.
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Who cites it
17 citing papers in PubMed.
- Connecting Nanoscale Molecular Self-Assembly to Macroscale Photophysical Property of Pyrene-Based Liquid Crystal Mesogen.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- High-throughput in situ sizing and quantum yield determination of individual perovskite nanocrystals.Nature materials · 2026Article
- Millisecond-Delayed Fluorescence in Heavy-Halogen-Substituted TADF Emitters for Air-Pressure Sensing.ACS applied materials & interfaces · 2026Article
- Vertically oriented 1D/3D heterojunction for efficient and stable inverted perovskite solar cells.Nature communications · 2026Article
- Machine learning for microscopy data analytics targeting real-time optical characterization of semiconductor nanocrystals.Nature communications · 2026Article
- Cryo-optical setup for wide-field microscopy and spectroscopy of luminescent nanomaterials.Nanoscale · 2026Article
- NIR Luminescence from Deep-Level Traps in CsPbBrThe journal of physical chemistry letters · 2025Article
- Extreme Electron-Photon Interaction in Disordered Perovskites.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Positive and Negative Effects under Light Illumination in Halide Perovskites.Small science · 2024Article
- 2D nanosheets of layered double perovskites: synthesis, photostable bright orange emission and photoluminescence blinking.Chemical science · 2023Article
- Self-Healing Ability of Perovskites Observed via Photoluminescence Response on Nanoscale Local Forces and Mechanical Damage.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2022Article
- The role of atmospheric conditions in the nonradiative recombination in individual CHNanoscale advances · 2022Article
- Manipulating crystallization dynamics through chelating molecules for bright perovskite emitters.Nature communications · 2021Article
- Article
- Are Shockley-Read-Hall and ABC models valid for lead halide perovskites?Nature communications · 2021Article
- Unveiling the Excited-State Dynamics of MnAdvanced science (Weinheim, Baden-Wurttemberg, Germany) · 2020Article
- Using Thermally Crosslinkable Hole Transporting Layer to Improve Interface Characteristics for Perovskite CsPbBrPolymers · 2020Article
Corrections and comments
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Authors and funding
9 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Organo-metal halide perovskites are promising solution-processed semiconductors, however, they possess diverse and largely not understood non-radiative mechanisms. Here, we resolve contributions of individual non-radiative recombination centers (quenchers) in nanocrystals of methylammonium lead iodide by studying their photoluminescence blinking caused by random switching of quenchers between active and passive states. We propose a model to describe the observed reduction of blinking upon cooling and determine energetic barriers of 0.2 to 0.8 eV for enabling the switching process, which points to ion migration as the underlying mechanism. Moreover, due to the strong influence of individual quenchers, the crystals show very individually-shaped photoluminescence enhancement upon cooling, suggesting that the high variety of activation energies of the PL enhancement reported in literature is not related to intrinsic properties but rather to the defect chemistry. Stabilizing the fluctuating quenchers in their passive states thus appears to be a promising strategy for improving the material quality.
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