Evidence map›Paper›PMID 30934165›Full record

ReviewAngewandte Chemie (International ed. in English)2019

Formation and Functioning of Bimetallic Nanocatalysts: The Power of X-ray Probes.

Matthias Filez, Evgeniy A Redekop, Jolien Dendooven, Ranjith K Ramachandran, Eduardo Solano, Unni Olsbye, Bert M Weckhuysen, Vladimir V Galvita, Hilde Poelman, Christophe Detavernier and 1 more

Abstract readReview
PubMed Full text at PMC Publisher
In one paragraph

Review in Angewandte Chemie (International ed. in English), 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.

0numbers the graph read from it
0cells of the map it votes in
6citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

6 citing papers in PubMed.

  1. Article
  2. Review
  3. Article
  4. Review
  5. Article
  6. Formation and Functioning of Bimetallic Nanocatalysts: The Power of X-ray Probes.Angewandte Chemie (International ed. in English) · 2019
    Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors.

Matthias FilezInorganic Chemistry and Catalysis group, Utrecht University, Universiteitsweg 99, 3584CG, Utrecht, The Netherlands.ORCID http://orcid.org/0000-0002-7810-637X
Evgeniy A RedekopCentre for Materials Science and Nanotechnology (SMN), Department of Chemistry, University of Oslo, P.O box 1126 Blindern, C0318, Oslo, Norway.ORCID http://orcid.org/0000-0001-6430-8811
Jolien DendoovenConformal Coatings of Nanomaterials group, Ghent University, Krijgslaan 281/S1, 9000, Ghent, Belgium.ORCID http://orcid.org/0000-0002-2385-3693
Ranjith K RamachandranConformal Coatings of Nanomaterials group, Ghent University, Krijgslaan 281/S1, 9000, Ghent, Belgium.
Eduardo SolanoConformal Coatings of Nanomaterials group, Ghent University, Krijgslaan 281/S1, 9000, Ghent, Belgium.
Unni OlsbyeCentre for Materials Science and Nanotechnology (SMN), Department of Chemistry, University of Oslo, P.O box 1126 Blindern, C0318, Oslo, Norway.
Bert M WeckhuysenInorganic Chemistry and Catalysis group, Utrecht University, Universiteitsweg 99, 3584CG, Utrecht, The Netherlands.ORCID http://orcid.org/0000-0001-5245-1426
Vladimir V GalvitaLaboratory for Chemical Technology, Ghent University, Technologiepark 125, 9052, Ghent, Belgium.ORCID http://orcid.org/0000-0001-9205-7917
Hilde PoelmanLaboratory for Chemical Technology, Ghent University, Technologiepark 125, 9052, Ghent, Belgium.
Christophe DetavernierConformal Coatings of Nanomaterials group, Ghent University, Krijgslaan 281/S1, 9000, Ghent, Belgium.ORCID http://orcid.org/0000-0001-7653-0858
Guy B MarinLaboratory for Chemical Technology, Ghent University, Technologiepark 125, 9052, Ghent, Belgium.ORCID http://orcid.org/0000-0002-6733-1213

Funding

Fonds Wetenschappelijk Onderzoek FWO postdoctoral fellowshipFonds Wetenschappelijk Onderzoek G.0209.11Fonds Wetenschappelijk Onderzoek Long Term Structural Methusalem Funding by the Flemish Government'FP7 Ideas: European Research Council FP7/2007-2013, No. 312284 (CALIPSO)H2020 Marie Skłodowska-Curie Actions 748563Nederlandse Organisatie voor Wetenschappelijk Onderzoek Gravitation Program MCEC (Multiscale Catalytic Energy Conversion)Norges Forskningsråd 272266
6 · The paper itself

Abstract

Bimetallic nanocatalysts are key enablers of current chemical technologies, including car exhaust converters and fuel cells, and play a crucial role in industry to promote a wide range of chemical reactions. However, owing to significant characterization challenges, insights in the dynamic phenomena that shape and change the working state of the catalyst await further refinement. Herein, we discuss the atomic-scale processes leading to mono- and bimetallic nanoparticle formation and highlight the dynamics and kinetics of lifetime changes in bimetallic catalysts with showcase examples for Pt-based systems. We discuss how in situ and operando X-ray spectroscopy, scattering, and diffraction can be used as a complementary toolbox to interrogate the working principles of today's and tomorrow's bimetallic nanocatalysts.

Indexed as

bimetallic nanocatalystscatalyst formationdeactivationX-ray characterization

Identifiers

PMID30934165
PMCPMC6771619

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.