ArticlePhilosophical transactions. Series A, Mathematical, physical, and engineering sciences2019
Ultrafast dynamics of spin and orbital correlations in quantum materials: an energy- and momentum-resolved perspective.
Article in Philosophical transactions. Series A, Mathematical, physical, and engineering sciences, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Ultrafast RIXS of orbital-resolved valence-band reshaping in photoexcited graphite.Science advances · 2026Article
- Ultrafast dynamics of vibronically dressed core excitons in graphite: a femtosecond RIXS perspective.Nature communications · 2025Article
- Development of a multi-functional chamber for resonant X-ray scattering experiments in the tender X-ray regime at the PAL-XFEL.Journal of synchrotron radiation · 2025Article
- Witnessing light-driven entanglement using time-resolved resonant inelastic X-ray scattering.Nature communications · 2023Article
- Laser-induced transient magnons in SrProceedings of the National Academy of Sciences of the United States of America · 2021Article
- The measurement of ultrafast electronic and structural dynamics with X-rays.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2019Article
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Authors and funding
7 authors.
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Abstract
Many remarkable properties of quantum materials emerge from states with intricate coupling between the charge, spin and orbital degrees of freedom. Ultrafast photo-excitation of these materials holds great promise for understanding and controlling the properties of these states. Here, we introduce time-resolved resonant inelastic X-ray scattering (tr-RIXS) as a means of measuring the charge, spin and orbital excitations out of equilibrium. These excitations encode the correlations and interactions that determine the detailed properties of the states generated. After outlining the basic principles and instrumentations of tr-RIXS, we review our first observations of transient antiferromagnetic correlations in quasi two dimensions in a photo-excited Mott insulator and present possible future routes of this fast-developing technique. The increasing number of X-ray free electron laser facilities not only enables tackling long-standing fundamental scientific problems, but also promises to unleash novel inelastic X-ray scattering spectroscopies. This article is part of the theme issue 'Measurement of ultrafast electronic and structural dynamics with X-rays'.
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