ArticleChemical science2019
A concentrated array of copper porphyrin candidate qubits.
Article in Chemical science, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 17 papers.
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Who cites it
17 citing papers in PubMed.
- Crystalline Small Molecule-Polymer Superlattice for Spatially Isolated Tetrathiafulvalene Spin Qubit Arrays.Angewandte Chemie (International ed. in English) · 2026Article
- Enlarging Quantum Coherence of Vanadyl Spin Qubits in Zirconium Porphyrinic MOFs.Inorganic chemistry · 2026Article
- Investigation of Hyperfine Interactions in Molecular Spin Qubits Constructed from A Nitronyl-Nitroxide Ligand and Transition Metal Ions.Inorganic chemistry · 2026Article
- Cerium-Based Metal-Organic Frameworks: Unveiling the Role of Terahertz Vibrations in the Spin Relaxation Dynamics.Inorganic chemistry · 2025Article
- Phononic modulation of spin-lattice relaxation in molecular qubit frameworks.Nature communications · 2024Article
- Spectroscopic Signatures of Phonon Character in Molecular Electron Spin Relaxation.ACS central science · 2024Article
- Stable organic radical qubits and their applications in quantum information science.Innovation (Cambridge (Mass.)) · 2024Review
- Weak Exchange Interactions in Multispin Systems: EPR Studies of Metalloporphyrins Decorated with {CrInorganic chemistry · 2024Article
- Motional Narrowing through Photonic Exchange: Rational Suppression of Excitonic Disorder from Molecular Cavity Polariton Formation.The journal of physical chemistry letters · 2024Article
- Determining the key vibrations for spin relaxation in ruffled Cu(ii) porphyrinsChemical science · 2024Article
- Decorrelated singlet and triplet exciton delocalization in acetylene-bridged Zn-porphyrin dimers.Chemical science · 2024Article
- Improving the molecular spin qubit performance in zirconium MOF composites by mechanochemical dilution and fullerene encapsulation.Chemical science · 2023Article
- Metal-organic frameworks as OChemical science · 2022Review
- Chemical control of spin-lattice relaxation to discover a room temperature molecular qubit.Chemical science · 2022Article
- Near IsotropicInorganic chemistry · 2021Article
- Probing Vibrational Symmetry Effects and Nuclear Spin Economy Principles in Molecular Spin Qubits.Inorganic chemistry · 2021Article
- Enhancing catalytic alkane hydroxylation by tuning the outer coordination sphere in a heme-containing metal-organic framework.Chemical science · 2020Article
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Authors and funding
5 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Synthetic chemistry offers a pathway to realize atomically precise arrays of qubits, the smallest unit of a quantum information science system. We harnessed framework chemistry to create an array of qubit candidates, featuring one qubit every 13.6 Å, by synthesizing the new copper(ii) variant of the porphyrinic metal-organic framework PCN-224. We subjected the framework to pulse-electron paramagnetic resonance (EPR) measurements, establishing spin coherence at temperatures up to 80 K within a fully spin concentrated framework. Observation of Rabi oscillations further support the viability of the qubits within these arrays. To interrogate the spin dynamics of qubit arrays, we investigated spin-lattice relaxation,
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