Evidence map›Paper›PMID 30742082›Full record

ArticleNature materials2019

Gate controlling of quantum interference and direct observation of anti-resonances in single molecule charge transport.

Yueqi Li, Marius Buerkle, Guangfeng Li, Ali Rostamian, Hui Wang, Zixiao Wang, David R Bowler, Tsuyoshi Miyazaki, Limin Xiang, Yoshihiro Asai and 2 more

Erratum issuedAbstract read
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In one paragraph

Article in Nature materials, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. An erratum has been issued. Cited by 43 papers.

0numbers the graph read from it
0cells of the map it votes in
43citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

43 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
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  5. Article
  6. Article
  7. Review
  8. Redox-Induced Atomic Switch as Platform for Molecular Electronics Devices.Small (Weinheim an der Bergstrasse, Germany) · 2025
    Article
  9. Article
  10. Article
  11. Article
  12. Article
  13. Single-Molecule Mechanoresistivity by Intermetallic Bonding.Angewandte Chemie (International ed. in English) · 2025
    Article
  14. Article
  15. Article
  16. Article
  17. Article
  18. Review
  19. Article
  20. Article
4 · The record

Corrections and comments

5 · Who and what money

Authors and funding

12 authors.

Yueqi LiBiodesign Center for Bioelectronics and Biosensors, Arizona State University, Tempe, AZ, USA.ORCID http://orcid.org/0000-0001-7003-1978
Marius BuerkleResearch Center for Computational Design of Advanced Functional Materials (CD-FMat), National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki, Japan.ORCID http://orcid.org/0000-0003-3464-2549
Guangfeng LiLaboratory of Advanced Materials, State Key Laboratory of Molecular Engineering of Polymers, Fudan University, Shanghai, China.
Ali RostamianBiodesign Center for Bioelectronics and Biosensors, Arizona State University, Tempe, AZ, USA.
Hui WangState Key Laboratory of Analytical Chemistry for Life Science, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, China.
Zixiao WangState Key Laboratory of Analytical Chemistry for Life Science, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, China.
David R BowlerLondon Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London, UK.ORCID http://orcid.org/0000-0001-7853-1520
Tsuyoshi MiyazakiInternational Centre for Materials Nanoarchitectonics (MANA), National Institute for Materials Science (NIMS) Tsukuba, Ibaraki, Japan.ORCID http://orcid.org/0000-0003-3534-4404
Limin XiangBiodesign Center for Bioelectronics and Biosensors, Arizona State University, Tempe, AZ, USA.
Yoshihiro AsaiResearch Center for Computational Design of Advanced Functional Materials (CD-FMat), National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki, Japan. yo-asai@aist.go.jp.ORCID http://orcid.org/0000-0003-4581-3921
Gang ZhouLaboratory of Advanced Materials, State Key Laboratory of Molecular Engineering of Polymers, Fudan University, Shanghai, China. zhougang@fudan.edu.cn.ORCID http://orcid.org/0000-0002-1533-7795
Nongjian TaoBiodesign Center for Bioelectronics and Biosensors, Arizona State University, Tempe, AZ, USA. nongjian.tao@asu.edu.ORCID http://orcid.org/0000-0002-5206-153X

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Quantum interference can profoundly affect charge transport in single molecules, but experiments can usually measure only the conductance at the Fermi energy. Because, in general, the most pronounced features of the quantum interference are not located at the Fermi energy, it is highly desirable to probe charge transport in a broader energy range. Here, by means of electrochemical gating, we measure the conductance and map the transmission functions of single molecules at and around the Fermi energy, and study signatures associated with constructive and destructive interference. With electrochemical gate control, we tune the quantum interference between the highest occupied molecular orbital and lowest unoccupied molecular orbital, and directly observe anti-resonance, a distinct feature of destructive interference. By tuning the molecule in and out of anti-resonance, we achieve continuous control of the conductance over two orders of magnitude with a subthreshold swing of ~17 mV dec

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.