ArticleACS nano2019
Coordination-Controlled C-C Coupling Products via ortho-Site C-H Activation.
Article in ACS nano, 2019. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- Stepwise on-surface synthesis of nitrogen-doped porous carbon nanoribbons.Communications chemistry · 2024Article
- Selective activation of four quasi-equivalent C-H bonds yields N-doped graphene nanoribbons with partial corannulene motifs.Nature communications · 2022Article
- Construction of heparin-based hydrogel incorporated with Cu5.4O ultrasmall nanozymes for wound healing and inflammation inhibition.Bioactive materials · 2021Article
- Polymerization of silanes through dehydrogenative Si-Si bond formation on metal surfaces.Nature chemistry · 2021Article
- Selective Intramolecular Dehydrocyclization of Co-Porphyrin on Au(111).Molecules (Basel, Switzerland) · 2020Article
- Snapshots of Dynamic Adaptation: Two-Dimensional Molecular Architectonics with Linear Bis-Hydroxamic Acid Modules.Angewandte Chemie (International ed. in English) · 2019Article
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Authors and funding
13 authors.
Funding
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Abstract
The coordination-restricted ortho-site C-H bond activation and dehydrogenative homocoupling of 4,4'-(1,3-phenylene)dipyridine (1,3-BPyB) and 4,4'-(1,4-phenylene)dipyridine (1,4-BPyB) on different metal surfaces were studied by a combination of scanning tunneling microscopy, noncontact atomic force microscopy, and density functional theory calculations. The coupling products on Cu(111) exhibited certain configurations subject to the spatial restriction of robust two-fold Cu-N coordination bonds. Compared to the V-shaped 1,3-BPyB, the straight backbone of 1,4-BPyB helped to further reduce the variety of reactive products. By utilizing the three-fold coordination of Fe atoms with 1,4-BPyB molecules on Au(111), a large-scale network containing single products was constructed. Our results offer a promising protocol for controllable on-surface synthesis with the aid of robust coordination interactions.
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