ArticleGels (Basel, Switzerland)2018
Chiral Assembly Preferences and Directing Effects in Supramolecular Two-Component Organogels.
Article in Gels (Basel, Switzerland), 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Understanding multicomponent low molecular weight gels from gelators to networks.Journal of advanced research · 2025Review
- Supramolecular Fractal Growth of Self-Assembled Fibrillar Networks.Gels (Basel, Switzerland) · 2021Article
- Using chirality to influence supramolecular gelation.Chemical science · 2019Article
- Diffusion across a gel-gel interface - molecular-scale mobility of self-assembled 'solid-like' gel nanofibres in multi-component supramolecular organogels.Chemical science · 2018Article
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Authors and funding
2 authors.
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Abstract
The impact of chirality on the self-assembly of supramolecular gels is of considerable importance, as molecular-scale programming can be translated into nanostructuring and ultimately affect macroscopic performance. This paper explores the effect of chirality on the assembly of two-component gels comprised of a second-generation dendritic lysine peptide acid, containing three chiral centres, and an amine. This combination forms an acid⁻amine complex that assembles into nanofibres through peptide-peptide hydrogen bonds, leading to organogels. With achiral amines, a racemic mixture of l,l,l and d,d,d dendritic peptide acids surprisingly forms the best gels-more commonly, mixing enantiomers suppresses gelation. Thermodynamic studies demonstrate that depending on the amine, the greater stability of heterochiral gels can either be entropically or enthalpically driven. With amines possessing "
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Registered trials
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