ArticleGels (Basel, Switzerland)2018
Relaxation Behavior by Time-Salt and Time-Temperature Superpositions of Polyelectrolyte Complexes from Coacervate to Precipitate.
Article in Gels (Basel, Switzerland), 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 18 papers.
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Who cites it
18 citing papers in PubMed.
- Effect of Copolymer Chemistry on the Humidity- and Temperature-Dependent Mechanical Properties and Structure of Polyelectrolyte Complexes.Macromolecules · 2026Article
- Enzyme-Induced Transition of the Morphology of Polyelectrolyte Complexes.Biomacromolecules · 2026Article
- Aqueous Processing of Stoichiometric and Nonstoichiometric Materials from Complex Coacervates.Accounts of materials research · 2025Article
- Role of Charge Patterning and Hydrophobicity in Peptide-Based Complex Coacervates.Biomacromolecules · 2025Article
- Unraveling the Temperature-Dependent Relaxation Dynamics of Ionic Liquid-Plasticized Compleximers.Macromolecules · 2025Article
- Cosolvent Control of Lower and Upper Critical Solution Behavior in Polyelectrolyte Complexes.ACS macro letters · 2025Article
- Effect of Cation-π Interactions on the Phase Behavior and Viscoelastic Properties of Polyelectrolyte Complexes.Macromolecules · 2025Article
- Brittle-to-Ductile Transitions of Polyelectrolyte Complexes: Humidity, Temperature, and Salt.Macromolecules · 2025Article
- Do Specific Ion Effects on Collective Relaxation Arise from Perturbation of Hydrogen-Bonding Network Structure?The journal of physical chemistry. B · 2024Article
- Counter Anion Type Influences the Glass Transition Temperature of Polyelectrolyte Complexes.Macromolecules · 2024Article
- Determinants of viscoelasticity and flow activation energy in biomolecular condensates.Science advances · 2024Article
- Effect of Dynamically Arrested Domains on the Phase Behavior, Linear Viscoelasticity and Microstructure of Hyaluronic Acid - Chitosan Complex Coacervates.Macromolecules · 2023Article
- Salt-Induced Diffusion of Star and Linear Polyelectrolytes within Multilayer Films.Macromolecules · 2023Article
- Role of dynamic bonds on fatigue threshold of tough hydrogels.Proceedings of the National Academy of Sciences of the United States of America · 2022Article
- Tuning the charge of polyelectrolyte complex membranes preparedSoft matter · 2021Article
- Polyelectrolyte Complex Membranes via Salinity Change Induced Aqueous Phase Separation.ACS applied polymer materials · 2020Article
- Characterization of the Ultralow Interfacial Tension in Liquid-Liquid Phase Separated Polyelectrolyte Complex Coacervates by the Deformed Drop Retraction Method.Macromolecules · 2019Article
- Lower Critical Solution Temperature in Polyelectrolyte Complex Coacervates.ACS macro letters · 2019Article
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2 authors.
Funding
Abstract
Complexation between anionic and cationic polyelectrolytes results in solid-like precipitates or liquid-like coacervate depending on the added salt in the aqueous medium. However, the boundary between these polymer-rich phases is quite broad and the associated changes in the polymer relaxation in the complexes across the transition regime are poorly understood. In this work, the relaxation dynamics of complexes across this transition is probed over a wide timescale by measuring viscoelastic spectra and zero-shear viscosities at varying temperatures and salt concentrations for two different salt types. We find that the complexes exhibit time-temperature superposition (TTS) at all salt concentrations, while the range of overlapped-frequencies for time-temperature-salt superposition (TTSS) strongly depends on the salt concentration (
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