ArticleScience advances2018
Multidimensional spectroscopy with attosecond extreme ultraviolet and shaped near-infrared pulses.
Article in Science advances, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
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Who cites it
6 citing papers in PubMed.
- A multidimensional approach to quantum state tomography of photoelectron wavepackets.Scientific reports · 2025Article
- All-fibre phase filters with 1-GHz resolution for high-speed passive optical logic processing.Nature communications · 2023Article
- Attosecond spectroscopy reveals alignment dependent core-hole dynamics in the ICl molecule.Nature communications · 2020Article
- Exploring the multiparameter nature of EUV-visible wave mixing at the FERMI FEL.Structural dynamics (Melville, N.Y.) · 2019Article
- Transient absorption spectroscopy using high harmonic generation: a review of ultrafast X-ray dynamics in molecules and solids.Philosophical transactions. Series A, Mathematical, physical, and engineering sciences · 2019Article
- IsoSense: frequency enhanced sensorless adaptive optics through structured illumination.Optica · 2019Article
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Authors and funding
4 authors.
Funding
Abstract
Dynamics following excitation with attosecond extreme ultraviolet (XUV) pulses arise from enormous numbers of accessible excited states, complicating the retrieval of state-specific time evolutions. We develop attosecond XUV multidimensional spectroscopy here to separate interfering pathways on a near-infrared (NIR) energy axis, retrieving single state dynamics in argon atoms in a two-dimensional (2D) XUV-NIR spectrum. In this experiment, we measure four-wave mixing signal arising from the interaction of XUV attosecond pulses centered around 15 eV with two few-cycle NIR pulses. The 2D spectrum is created by measuring the emitted XUV signal field spectrum while applying narrowband amplitude and phase modulations to one of the NIR pulses. Application of such a technique to systems of high dimensionality will provide for the observation of state-resolved pure electronic dynamics, in direct analogy to phenomena unraveled by multidimensional spectroscopies at optical frequencies.
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Registered trials
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