ArticleInternational journal of molecular sciences2018
Effect of Central Longitudinal Dipole Interactions on Chiral Liquid-Crystal Phases.
Article in International journal of molecular sciences, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Monte Carlo simulations of chiral liquid-crystals, represented by a simple coarse-grained chiral Gay⁻Berne model, were performed to investigate the effect of central longitudinal dipole interactions on phase behavior. A systematic analysis of the structural properties and phase behavior of both achiral and chiral systems, with dipole interactions, reveals differing effects; strong dipole interactions enhance the formation of layered structures; however, chiral interactions may prevent the formation of such phases under certain conditions. We also observed a short-ranged smectic structure within the cholesteric phases with strong dipole interactions. This constitutes possible evidence of presmectic ordering and/or the existence of chiral line liquid phases, which have previously been observed in X-ray experiments to occur between the smectic twisted grain boundary and cholesteric phases. These results provide a systematic understanding of how the phase behavior of chiral liquid-crystals changes when alterations are made to the strength of dipole interactions.
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