ArticleScientific reports2018
Dynamic multistimuli-responsive reversible chiral transformation in supramolecular helices.
Article in Scientific reports, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Dynamic Olefinic Bond Restructuring in Coordination Polymers Enables Precision Photocycloaddition.Chemistry (Weinheim an der Bergstrasse, Germany) · 2026Article
- Multivalent-Anion-Induced Inversion of Chiroptical Signals in a Cyanine Dye Bound to Nanotubular Supramolecular Assemblies.Langmuir : the ACS journal of surfaces and colloids · 2026Article
- Self-Regulating Hydrogel with Reversible Optical Activity in Its Gel-to-Gel Transformation.Journal of the American Chemical Society · 2025Article
- Responsive Supramolecular Polymers for Diagnosis and Treatment.International journal of molecular sciences · 2024Review
- Reversible chirality inversion of an AuAgNature communications · 2024Article
- Uncovering supramolecular chirality codes for the design of tunable biomaterials.Nature communications · 2024Article
- Programmable supramolecular chirality in non-equilibrium systems affording a multistate chiroptical switch.Nature communications · 2023Article
- Polarization-induced nanohelixes of organic cocrystals from asymmetric components with dopant-induced chirality inversion.Chemical science · 2023Article
- Chirality at nanoscale for bioscience.Chemical science · 2022Review
- An Azobenzene-Based Single-Component Supramolecular Polymer Responsive to Multiple Stimuli in Water.Journal of the American Chemical Society · 2020Article
- Meet the Board ofChemistryOpen · 2019Article
- Chiral nanostructures self-assembled from nitrocinnamic amide amphiphiles: substituent and solvent effects.Beilstein journal of nanotechnology · 2019Article
Corrections and comments
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Authors and funding
8 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The design of new chiral chromophores that allow tunable assembly of higher order helical structures by using natural stimuli offers promising avenue in understanding various biological processes. In particular, access to dynamic multistimuli-responsive systems can provide real-time monitoring of chiral transformation in chemical and biological systems. We report on the synthesis of naphthalenediimide appended L-glutamate (NDI-L-Glu) that self-assembles into chiral supramolecular structures under physiological conditions. Specifically, NDI-L-Glu shows a mixture of left- and right-handed helices under physiological conditions, and any deviation from the ambient biochemical environment has a remarkable influence on the chirality of these structures. For instance, acidic environments shift the helicity to left-handedness while the alkaline conditions reversed the helical structures to right-handedness, thereby mimicking the molecular virulence mechanism of tobacco mosaic virus (TMV). The chirality of these supramolecular assemblies can also be controllably tuned by using temperature as an external stimulus, allowing reversible flip of helicity.
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Registered trials
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