ArticleScientific reports2018
Energy transfer and correlations in cavity-embedded donor-acceptor configurations.
Article in Scientific reports, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed.
- Cavity-enhanced energy transport in molecular systems.Nature materials · 2025Review
- The Rise and Current Status of Polaritonic Photochemistry and Photophysics.Chemical reviews · 2023Review
- Theoretical Analysis of Exciton Wave Packet Dynamics in Polaritonic Wires.The journal of physical chemistry letters · 2023Article
- Simulating molecular polaritons in the collective regime using few-molecule models.Proceedings of the National Academy of Sciences of the United States of America · 2023Article
- Polariton chemistry: Thinking inside the (photon) box.Proceedings of the National Academy of Sciences of the United States of America · 2019Article
- Modification of excitation and charge transfer in cavity quantum-electrodynamical chemistry.Proceedings of the National Academy of Sciences of the United States of America · 2019Article
- Coherent Light Harvesting through Strong Coupling to Confined Light.The journal of physical chemistry letters · 2018Article
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Authors and funding
3 authors.
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Abstract
The rate of energy transfer in donor-acceptor systems can be manipulated via the common interaction with the confined electromagnetic modes of a micro-cavity. We analyze the competition between the near-field short range dipole-dipole energy exchange processes and the cavity mediated long-range interactions in a simplified model consisting of effective two-level quantum emitters that could be relevant for molecules in experiments under cryogenic conditions. We find that free-space collective incoherent interactions, typically associated with sub- and superradiance, can modify the traditional resonant energy transfer scaling with distance. The same holds true for cavity-mediated collective incoherent interactions in a weak-coupling but strong-cooperativity regime. In the strong coupling regime, we elucidate the effect of pumping into cavity polaritons and analytically identify an optimal energy flow regime characterized by equal donor/acceptor Hopfield coefficients in the middle polariton. Finally we quantify the build-up of quantum correlations in the donor-acceptor system via the two-qubit concurrence as a measure of entanglement.
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