ArticleNature communications2018
Transient modes of zeolite surface growth from 3D gel-like islands to 2D single layers.
Article in Nature communications, 2018. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 16 papers.
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Who cites it
16 citing papers in PubMed.
- To seed or not to seed? That is the question for zeolite AFI crystallization.Chemical science · 2026Article
- Split Syntheses: Introducing Bottom-Up Control over Aluminum in SSZ-13 and ZSM-5 Zeolites.JACS Au · 2025Article
- Triboelectric nanogenerator based on silane-coupled LTA/PDMS for physiological monitoring and biomechanical energy harvesting.Microsystems & nanoengineering · 2024Article
- Dynamic imaging of interfacial electrochemistry on single Ag nanowires by azimuth-modulated plasmonic scattering interferometry.Nature communications · 2023Article
- In Situ Multinuclear Magic-Angle Spinning NMR: Monitoring Crystallization of Molecular Sieve AlPOJACS Au · 2023Article
- Impact of a polymer modifier on directing the non-classical crystallization pathway of TS-1 zeolite: accelerating nucleation and enriching active sites.Chemical science · 2022Article
- Nucleation of Porous Crystals from Ion-Paired Prenucleation Clusters.Chemistry of materials : a publication of the American Chemical Society · 2022Article
- Time-resolved dissolution elucidates the mechanism of zeolite MFI crystallization.Science advances · 2021Article
- Discovering Relationships between OSDAs and Zeolites through Data Mining and Generative Neural Networks.ACS central science · 2021Article
- In situ imaging of two-dimensional surface growth reveals the prevalence and role of defects in zeolite crystallization.Proceedings of the National Academy of Sciences of the United States of America · 2020Article
- Structural and electronic switching of a single crystal 2D metal-organic framework prepared by chemical vapor deposition.Nature communications · 2020Article
- Minerals from colloidal assembly.Nature materials · 2020Article
- Tracking the rearrangement of atomic configurations during the conversion ofChemical science · 2019Article
- Influence of alkalinity on the synthesis of hierarchical LTA zeolite by using bridged polysilsesquioxane.RSC advances · 2019Article
- Uniformly Oriented Zeolite ZSM-5 Membranes with Tunable Wettability on a Porous Ceramic.Angewandte Chemie (International ed. in English) · 2018Article
- Nuclear Magnetic Resonance Spectroscopy for In Situ Monitoring of Porous Materials Formation under Hydrothermal Conditions.Materials (Basel, Switzerland) · 2018Review
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Authors and funding
3 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Zeolite crystallization occurs by multifaceted processes involving molecule attachment and nonclassical pathways governed by the addition of amorphous precursors. Here, we use scanning probe microscopy to monitor zeolite LTA crystallization in situ with a spatiotemporal resolution that captures dynamic processes in real time. We report a distinctive pathway involving the formation of gel-like islands from supersaturated solutions comprised of (alumino)silicate molecules. Three-dimensional assembly and evolution of these islands constitutes a unique mode of growth that differs from classical theories. Time-resolved imaging also reveals that growth can occur by (nearly) oriented attachment. At later stages of crystallization, a progressive transition to lower supersaturation shifts growth to a layered mechanism involving two-dimensional nucleation and spreading of layers. Here, we show that LTA crystallization occurs by multiple pathways, thereby reconciling putative hypotheses of growth mechanisms while also highlighting new modes of nonclassical crystallization that may prove relevant to other zeolites and related materials.
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